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Linking meteorology, turbulence, and air chemistry in the amazon rain forest
Fuentes, José D.; Chamecki, Marcelo; dos Santos, Rosa Maria Nascimento; Von Randow, Celso; Stoy, Paul C.; Katul, Gabriel George; Fitzjarrald, David RoyA field campaign reveals that the Amazon rain forest produces enough chemical species to undergo oxidation and generate aerosols, which can activate into cloud condensation nuclei and potentially influence cloud formation. © 2016 American Meteorological Society.
Dimethyl sulfide in the Amazon rain forest
Jardine, Kolby J.; Yáñez-Serrano, Ana Maria; Williams, Jonathan C.; Kunert, Norbert; Jardine, Angela B.; Taylor, Tyeen C.; Abrell, Leif; Artaxo, PauloSurface-to-atmosphere emissions of dimethyl sulfide (DMS) may impact global climate through the formation of gaseous sulfuric acid, which can yield secondary sulfate aerosols and contribute to new particle formation. While oceans are generally considered the dominant sources of DMS, a shortage of ecosystem observations prevents an accurate analysis of terrestrial DMS sources. Using mass spectrometry, we quantif...
Highly reactive light-dependent monoterpenes in the Amazon
Jardine, Angela B.; Jardine, Kolby J.; Fuentes, José D.; Martin, Scot T.; Martins, Giordane Augusto; Durgante, Flávia MachadoDespite orders of magnitude difference in atmospheric reactivity and great diversity in biological functioning, little is known about monoterpene speciation in tropical forests. Here we report vertically resolved ambient air mixing ratios for 12 monoterpenes in a central Amazon rainforest including observations of the highly reactive cis-β-ocimene (160 ppt), trans-β-ocimene (79 ppt), and terpinolene (32 ppt) wh...
Dynamic balancing of isoprene carbon sources reflects photosynthetic and photor...
Jardine, Kolby J.; Chambers, Jeffrey Quintin; Alves, Eliane Gomes; Teixeira, Andrea; Garcia, Sabrina; Holm, Jennifer A.; Higuchi, NiroThe volatile gas isoprene is emitted in teragrams per annum quantities from the terrestrial biosphere and exerts a large effect on atmospheric chemistry. Isoprene is made primarily from recently fixed photosynthate; however, alternate carbon sources play an important role, particularly when photosynthate is limiting. We examined the relative contribution of these alternate carbon sources under changes in light ...
Urban pollution greatly enhances formation of natural aerosols over the Amazon ...
Shrivastava, Manish K.; Andreae, Meinrat O.; Artaxo, Paulo; Barbosa, H. M. J.; Berg, Larry K.; Brito, Joel F.; Ching, Joseph; Easter, Richard C.One of the least understood aspects in atmospheric chemistry is how urban emissions influence the formation of natural organic aerosols, which affect Earth’s energy budget. The Amazon rainforest, during its wet season, is one of the few remaining places on Earth where atmospheric chemistry transitions between preindustrial and urban-influenced conditions. Here, we integrate insights from several laboratory meas...