Thiswork introduces theencapsulationofhexamethylenediisocyanatederivatives(HDI,TriHDI, andPHDI)with thebiodegradablepolymerpoly(butyleneadipate-co-terephthalate) (PBAT) through a solvent evaporationmethod. Thesemicrocapsules(MCs)werethenemployedinadhesiveformulations for footwear.Moreover,MCs containingPHDIwereproduced ina closed vessel, demonstrating the potential for recovering and reusingorganicsolventsforth...