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Bifunctional atomically dispersed ruthenium electrocatalysts for efficient bipo...
Yu, Zhipeng; Si, Chaowei; Escobar-Bedia, Francisco Javier; LaGrow, Alec P.; Xu, Junyuan; Sabater, Maria J.; Amorim, Isilda; Araujo, AnaAtomically dispersed catalysts (ADCs) have recently drawn considerable interest for use in water electrolysis to produce hydrogen, because they allow for maximal utilization of metal species, particularly the expensive and scarce platinum group metals. Herein, we report the electrocatalytic performance of atomically dispersed ruthenium catalysts (Ru ADCs) with ultralow Ru loading (0.2 wt%). The as-obtained Ru A...
Iridium–Iron Diatomic Active Sites for Efficient Bifunctional Oxygen Electrocat...
Yu, Zhipeng; Si, Chaowei; LaGrow, Alec P.; Tai, Zhixin; Caliebe, Wolfgang A.; Tayal, Akhil; Sampaio, Maria J.; Sousa, Juliana P. S.; Amorim, IsildaDiatomic catalysts, particularly those with heteronuclear active sites, have recently attracted considerable attention for their advantages over single-atom catalysts in reactions involving multielectron transfers. Herein, we report bimetallic iridium−iron diatomic catalysts (IrFe−N−C) derived from metal−organic frameworks in a facile wet chemical synthesis followed by postpyrolysis. We use various advanced cha...