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Multifunctional hard coatings based on CrNx for temperature sensing applications

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Resumo:This paper presents reports on the preparation of a multifunctional coating system, CrNx, with temperature sensing capability. A systematic study of the thermo-resistive effect of chromium nitride (CrNx) thin films with a negative temperature coefficient of resistance (TCR) has been carried out. The CrNx nanostructures were grown by reactive magnetron sputtering under distinct Ar+N2 conditions. To confer a zigzag columnar morphology to the CrNx we explored the oblique angle deposition technique. The structural properties have been studied through X-ray diffraction and Scanning Electron Microscopy. The thermo-resistive response was evaluated by measuring the electrical resistivity as a function of temperature by the twopoint method. The results observed for the CrNx films produced with N2 flux between 4 and 8 sccm present an stable and negative TCR. Values of -9.1710-4 , -5.3110-3 , and -1.47610-2 were observed for the films grown with 4, 6, and 8 sccm, respectively. The grain-boundary was used to theoretically describe our results. The results open new technological possibilities for the application of CrNx coatings for esistive temperature detector (RTD) systems.
Autores principais:Ferreira, Armando José Barros
Outros Autores:Correa, Marcio A.; Silva, João Paulo; Correia, Daniela Maria Silva; Lanceros-Méndez, S.; Vaz, F.
Assunto:Multifunctional hard coatings DC sputtering Temperature Coefficient of Resistance Thermal properties Temperature sensing
Ano:2021
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso restrito
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:This paper presents reports on the preparation of a multifunctional coating system, CrNx, with temperature sensing capability. A systematic study of the thermo-resistive effect of chromium nitride (CrNx) thin films with a negative temperature coefficient of resistance (TCR) has been carried out. The CrNx nanostructures were grown by reactive magnetron sputtering under distinct Ar+N2 conditions. To confer a zigzag columnar morphology to the CrNx we explored the oblique angle deposition technique. The structural properties have been studied through X-ray diffraction and Scanning Electron Microscopy. The thermo-resistive response was evaluated by measuring the electrical resistivity as a function of temperature by the twopoint method. The results observed for the CrNx films produced with N2 flux between 4 and 8 sccm present an stable and negative TCR. Values of -9.1710-4 , -5.3110-3 , and -1.47610-2 were observed for the films grown with 4, 6, and 8 sccm, respectively. The grain-boundary was used to theoretically describe our results. The results open new technological possibilities for the application of CrNx coatings for esistive temperature detector (RTD) systems.