Publicação

Structure-property relationships in push-pull amino/cyanovinyl end-capped oligothiophenes : quantum chemical and experimental studies

Ver documento

Detalhes bibliográficos
Resumo:A series of push-pull chromophores built around thiophene-based π-conjugating spacers and bearing various types of amino-donors and cyanovinyl-acceptors have been analysed by means of UV-Vis-NIR, IR and Raman spectroscopic measurements in the solid state as well as in solution. The intramolecular charge transfer (ICT) of these π-conjugated systems has also been tested by analysing the ability of the solute molecules in undergoing shifts in their fluorescence emission maxima with increasing solvent polarity. These push-pull oligomers also display an attractive electrochemical behaviour since they generate stable species both upon oxidation and reduction. Oxidation mainly involves changes in the electron-rich aminooligothienyl half-part of the molecule and leads to the formation of stable cations. On the other hand, reduction to radical anions and dianions is mainly cyanovinyl-centered but also affects the π-conjugated electron-relay. Density functional theory (DFT) calculations have been carried out to help the assignment of the most relevant electronic and vibrational features and to derive useful information about the molecular structure of these NLO-phores.
Autores principais:Oliva, María Moreno
Outros Autores:Casado, Juan; Raposo, M. Manuela M.; Fonseca, A. Maurício C.; Hartmann, Horst; Hernández, Víctor; Navarrete, Juan T. López
Assunto:Thiophene Push-pull oligomers Dicyanovinyl heterocycles Electronic structure DFT calculations Electrochemical properties Nonlinear optical (NLO) materials Oligothiophenes Ciências Naturais::Ciências Químicas
Ano:2006
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso restrito
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:A series of push-pull chromophores built around thiophene-based π-conjugating spacers and bearing various types of amino-donors and cyanovinyl-acceptors have been analysed by means of UV-Vis-NIR, IR and Raman spectroscopic measurements in the solid state as well as in solution. The intramolecular charge transfer (ICT) of these π-conjugated systems has also been tested by analysing the ability of the solute molecules in undergoing shifts in their fluorescence emission maxima with increasing solvent polarity. These push-pull oligomers also display an attractive electrochemical behaviour since they generate stable species both upon oxidation and reduction. Oxidation mainly involves changes in the electron-rich aminooligothienyl half-part of the molecule and leads to the formation of stable cations. On the other hand, reduction to radical anions and dianions is mainly cyanovinyl-centered but also affects the π-conjugated electron-relay. Density functional theory (DFT) calculations have been carried out to help the assignment of the most relevant electronic and vibrational features and to derive useful information about the molecular structure of these NLO-phores.