Publicação

Unzipping of functionalized multiwall carbon nanotubes Induced by STM

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Detalhes bibliográficos
Resumo:Carbon nanotubes (CNTs), functionalized by a cycloaddition reaction, were studied by ultrahigh vacuum scanning tunneling microscopy (STM). The STM images provided evidence for partial or total unzipping of the outer CNT layer. The formation of graphene ribbons was triggered by the STM tip, under specific operating conditions. A model for the unzipping is proposed, based on the perturbation of the π-conjugation along the CNT surface induced by the cycloaddition reaction.
Autores principais:Paiva, M. C.
Outros Autores:Xu, Wei; Proença, M. Fernanda R. P.; Novais, R. M.; Laegsgaard, E.; Besenbacher, F.
Assunto:Carbon nanotube Graphene Cycloaddition reaction Scanning tunneling microscopy Grapheme
Ano:2010
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso restrito
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:Carbon nanotubes (CNTs), functionalized by a cycloaddition reaction, were studied by ultrahigh vacuum scanning tunneling microscopy (STM). The STM images provided evidence for partial or total unzipping of the outer CNT layer. The formation of graphene ribbons was triggered by the STM tip, under specific operating conditions. A model for the unzipping is proposed, based on the perturbation of the π-conjugation along the CNT surface induced by the cycloaddition reaction.