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Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils

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Resumo:The volatile and olfactory profiles of three Portuguese olive oils with protected designations of origin (PDO) were studied: "Azeite do Alentejo Interior", "Azeites da Beira Interior", and "Azeite de Tras-os-Montes". Seven classes of volatiles were identified, with aldehydes, followed by hydrocarbons and alcohols, the most prevalent (5.63, 2.92, and 2.79 mg/kg olive oil, respectively). The "Azeites da Beira Interior" oils exhibited the highest amount of volatiles (18.2 +/- 4.6 mg/kg olive oil) compared to the oils from the other two PDOs. Ten positive olfactory sensations were detected, and a significant effect of the PDO on the intensities of fruity, apple, cabbage, tomato, dry and fresh herbs was observed. Specifically, "Azeite do Alentejo Interior" PDO oils were characterized as fruity-ripe, while "Azeite de Tras-os-Montes" PDO oils were labelled as fruity-green. Conversely, "Azeites da Beira Interior" PDO oils encompassed both fruity-ripe and fruity-green oils. Unique volatile and olfactory fingerprints were established for each PDO, allowing the linear discrimination of the oils according to the PDO, with a predictive sensitivity of 98.0 +/- 4.2% (repeated K-fold-CV). Furthermore, a lab-made electronic nose successfully discriminated the studied oils based on the PDO, with a predictive accuracy of 99.7 +/- 2.0% (repeated K-fold-CV). This device also allowed predicting the concentrations of the three main volatile classes found in the oils through multiple linear regression models (R2 >= 0.923 +/- 0.101 and RMSE <= 1.32 +/- 0.72 mg/kg oil; repeated K-fold-CV). These findings underscore the potential of the electronic nose as a reliable traceability tool to authenticate the PDO declaration of Portuguese olive oils, and broaden its use beyond non-PDO oils from a specific geographical area to encompass a national scale.
Autores principais:Rodrigues, Nuno
Outros Autores:Ferreiro, Nuno Manuel; Ruano, Daniela Filipa Magalhães; Dias, Francisco; Veloso, Ana C.A.; Pereira, J.A.; Peres, António M.
Assunto:Chemometrics Geographical origin Gas sensors Sensory panel Volatile profile
Ano:2024
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Instituto Politécnico de Bragança
Idioma:inglês
Origem:Biblioteca Digital do IPB
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author Rodrigues, Nuno
author2 Ferreiro, Nuno Manuel
Ruano, Daniela Filipa Magalhães
Dias, Francisco
Veloso, Ana C.A.
Pereira, J.A.
Peres, António M.
author2_role author
author
author
author
author
author
author_facet Rodrigues, Nuno
Ferreiro, Nuno Manuel
Ruano, Daniela Filipa Magalhães
Dias, Francisco
Veloso, Ana C.A.
Pereira, J.A.
Peres, António M.
author_role author
contributor_name_str_mv Biblioteca Digital do IPB
country_str PT
creators_json_txt [{\"Person.name\":\"Rodrigues, Nuno\",\"Person.identifier.orcid\":\"0000-0002-9305-0976\"},{\"Person.name\":\"Ferreiro, Nuno Manuel\"},{\"Person.name\":\"Ruano, Daniela Filipa Magalhães\"},{\"Person.name\":\"Dias, Francisco\"},{\"Person.name\":\"Veloso, Ana C.A.\"},{\"Person.name\":\"Pereira, J.A.\",\"Person.identifier.orcid\":\"0000-0002-2260-0600\"},{\"Person.name\":\"Peres, António M.\",\"Person.identifier.orcid\":\"0000-0001-6595-9165\"}]
datacite.contributors.contributor.contributorName.fl_str_mv Biblioteca Digital do IPB
datacite.creators.creator.creatorName.fl_str_mv Rodrigues, Nuno
Ferreiro, Nuno Manuel
Ruano, Daniela Filipa Magalhães
Dias, Francisco
Veloso, Ana C.A.
Pereira, J.A.
Peres, António M.
datacite.date.Accepted.fl_str_mv 2024-01-01T00:00:00Z
datacite.date.available.fl_str_mv 2024-05-14T09:16:04Z
datacite.date.embargoed.fl_str_mv 2024-05-14T09:16:04Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv Chemometrics
Geographical origin
Gas sensors
Sensory panel
Volatile profile
datacite.titles.title.fl_str_mv Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
dc.contributor.none.fl_str_mv Biblioteca Digital do IPB
dc.creator.none.fl_str_mv Rodrigues, Nuno
Ferreiro, Nuno Manuel
Ruano, Daniela Filipa Magalhães
Dias, Francisco
Veloso, Ana C.A.
Pereira, J.A.
Peres, António M.
dc.date.Accepted.fl_str_mv 2024-01-01T00:00:00Z
dc.date.available.fl_str_mv 2024-05-14T09:16:04Z
dc.date.embargoed.fl_str_mv 2024-05-14T09:16:04Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv http://hdl.handle.net/10198/29764
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv Springer
dc.rights.cclincense.fl_str_mv http://creativecommons.org/licenses/by/4.0/
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.subject.none.fl_str_mv Chemometrics
Geographical origin
Gas sensors
Sensory panel
Volatile profile
dc.title.fl_str_mv Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_6501
description The volatile and olfactory profiles of three Portuguese olive oils with protected designations of origin (PDO) were studied: "Azeite do Alentejo Interior", "Azeites da Beira Interior", and "Azeite de Tras-os-Montes". Seven classes of volatiles were identified, with aldehydes, followed by hydrocarbons and alcohols, the most prevalent (5.63, 2.92, and 2.79 mg/kg olive oil, respectively). The "Azeites da Beira Interior" oils exhibited the highest amount of volatiles (18.2 +/- 4.6 mg/kg olive oil) compared to the oils from the other two PDOs. Ten positive olfactory sensations were detected, and a significant effect of the PDO on the intensities of fruity, apple, cabbage, tomato, dry and fresh herbs was observed. Specifically, "Azeite do Alentejo Interior" PDO oils were characterized as fruity-ripe, while "Azeite de Tras-os-Montes" PDO oils were labelled as fruity-green. Conversely, "Azeites da Beira Interior" PDO oils encompassed both fruity-ripe and fruity-green oils. Unique volatile and olfactory fingerprints were established for each PDO, allowing the linear discrimination of the oils according to the PDO, with a predictive sensitivity of 98.0 +/- 4.2% (repeated K-fold-CV). Furthermore, a lab-made electronic nose successfully discriminated the studied oils based on the PDO, with a predictive accuracy of 99.7 +/- 2.0% (repeated K-fold-CV). This device also allowed predicting the concentrations of the three main volatile classes found in the oils through multiple linear regression models (R2 >= 0.923 +/- 0.101 and RMSE <= 1.32 +/- 0.72 mg/kg oil; repeated K-fold-CV). These findings underscore the potential of the electronic nose as a reliable traceability tool to authenticate the PDO declaration of Portuguese olive oils, and broaden its use beyond non-PDO oils from a specific geographical area to encompass a national scale.
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Fundação para a Ciência e a Tecnologia
Fundação para a Ciência e a Tecnologia
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person_str_mv Rodrigues, Nuno
Rodrigues, Nuno
https://www.ciencia-id.pt/F41D-B424-5F78
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Ferreiro, Nuno Manuel
Ruano, Daniela Filipa Magalhães
Dias, Francisco
Veloso, Ana C.A.
Pereira, J.A.
Pereira, J.A.
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publisher.none.fl_str_mv Springer
reponame_str Biblioteca Digital do IPB
repository_id_str urn:repositoryAcronym:ipb
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spelling engSpringerpt_PTThe volatile and olfactory profiles of three Portuguese olive oils with protected designations of origin (PDO) were studied: "Azeite do Alentejo Interior", "Azeites da Beira Interior", and "Azeite de Tras-os-Montes". Seven classes of volatiles were identified, with aldehydes, followed by hydrocarbons and alcohols, the most prevalent (5.63, 2.92, and 2.79 mg/kg olive oil, respectively). The "Azeites da Beira Interior" oils exhibited the highest amount of volatiles (18.2 +/- 4.6 mg/kg olive oil) compared to the oils from the other two PDOs. Ten positive olfactory sensations were detected, and a significant effect of the PDO on the intensities of fruity, apple, cabbage, tomato, dry and fresh herbs was observed. Specifically, "Azeite do Alentejo Interior" PDO oils were characterized as fruity-ripe, while "Azeite de Tras-os-Montes" PDO oils were labelled as fruity-green. Conversely, "Azeites da Beira Interior" PDO oils encompassed both fruity-ripe and fruity-green oils. Unique volatile and olfactory fingerprints were established for each PDO, allowing the linear discrimination of the oils according to the PDO, with a predictive sensitivity of 98.0 +/- 4.2% (repeated K-fold-CV). Furthermore, a lab-made electronic nose successfully discriminated the studied oils based on the PDO, with a predictive accuracy of 99.7 +/- 2.0% (repeated K-fold-CV). This device also allowed predicting the concentrations of the three main volatile classes found in the oils through multiple linear regression models (R2 >= 0.923 +/- 0.101 and RMSE <= 1.32 +/- 0.72 mg/kg oil; repeated K-fold-CV). These findings underscore the potential of the electronic nose as a reliable traceability tool to authenticate the PDO declaration of Portuguese olive oils, and broaden its use beyond non-PDO oils from a specific geographical area to encompass a national scale.application/pdfpt_PTElectronic nose: a tool to verify the PDO declaration of Portuguese olive oilsPersonalRodrigues, NunoDSpacehttp://dspace.org/items/00739d63-995d-4b1f-97d0-03d24c7cf0fdDSpacehttp://dspace.org/items/00739d63-995d-4b1f-97d0-03d24c7cf0fdRodriguesNunoCiência IDhttps://www.ciencia-id.ptF41D-B424-5F78ORCIDhttp://orcid.org0000-0002-9305-0976Scopus Author IDhttps://www.scopus.com55258560600Ferreiro, Nuno ManuelRuano, Daniela Filipa MagalhãesDias, FranciscoVeloso, Ana C.A.PersonalPereira, J.A.DSpacehttp://dspace.org/items/7932162e-a2da-4913-b00d-17babbe51857DSpacehttp://dspace.org/items/7932162e-a2da-4913-b00d-17babbe51857PereiraJosé AlbertoCiência IDhttps://www.ciencia-id.pt611F-80B2-A7C1ORCIDhttp://orcid.org0000-0002-2260-0600Researcher IDhttps://www.researcherid.comL-6798-2014Scopus Author IDhttps://www.scopus.com57204366348PersonalPeres, António M.DSpacehttp://dspace.org/items/7d93be47-8dc4-4413-9304-5b978773d3bbDSpacehttp://dspace.org/items/7d93be47-8dc4-4413-9304-5b978773d3bbPeresAntónio M.Ciência IDhttps://www.ciencia-id.ptCF16-5443-F420ORCIDhttp://orcid.org0000-0001-6595-9165Researcher IDhttps://www.researcherid.comI-8470-2012Scopus Author IDhttps://www.scopus.com7102331969HostingInstitutionOrganizationalBiblioteca Digital do IPBe-mailmailto:dspace@ipb.ptdspace@ipb.ptISSNIsPartOf2193-4126DOIIsPartOf10.1007/s11694-024-02374-42024-05-14T09:16:04Z20242024-01-01T00:00:00ZHandlehttp://hdl.handle.net/10198/29764http://purl.org/coar/access_right/c_abf2open accessChemometricsGeographical originGas sensorsSensory panelVolatile profile1766409 bytesFundação para a Ciência e a TecnologiaMountain Research Center6817 - DCRRNI IDCrossref Funder IDhttp://doi.org/10.13039/501100001871Fundação para a Ciência e a TecnologiaMountain Research Center6817 - DCRRNI IDCrossref Funder IDhttp://doi.org/10.13039/501100001871Fundação para a Ciência e a TecnologiaCentre of Biological Engineering of the University of Minho6817 - DCRRNI IDCrossref Funder IDhttp://doi.org/10.13039/501100001871Fundação para a Ciência e a TecnologiaAssociate Laboratory for Sustainability and Tecnology in Mountain Regions6817 - DCRRNI IDCrossref Funder IDhttp://doi.org/10.13039/501100001871Fundação para a Ciência e a TecnologiaExtra virgin olive oil shelf-life prediction based on an integrated approach from farm to forkPOR_NORTECrossref Funder IDhttp://doi.org/10.13039/501100001871literaturehttp://purl.org/coar/resource_type/c_6501journal article2024http://creativecommons.org/licenses/by/4.0/http://purl.org/coar/access_right/c_abf2application/pdffulltexthttps://bibliotecadigital.ipb.pt/bitstreams/f4a48c16-0e87-4941-84c3-606a75d30d06/downloadJournal of Food Measurement and Characterization18429522964
spellingShingle Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
Rodrigues, Nuno
Chemometrics
Geographical origin
Gas sensors
Sensory panel
Volatile profile
status SINGLETON
subject.fl_str_mv Chemometrics
Geographical origin
Gas sensors
Sensory panel
Volatile profile
title Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
title_full Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
title_fullStr Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
title_full_unstemmed Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
title_short Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
title_sort Electronic nose: a tool to verify the PDO declaration of Portuguese olive oils
topic Chemometrics
Geographical origin
Gas sensors
Sensory panel
Volatile profile
topic_facet Chemometrics
Geographical origin
Gas sensors
Sensory panel
Volatile profile
url http://hdl.handle.net/10198/29764
visible 1