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Detection of botanical adulterations in plant food supplements by molecular biology techniques

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Resumo:In the last years, botanicals have become increasingly available in the EU market in the form of plant food supplements (PFS), which are legally considered as foods under Directive 2002/46/EC and consequently not submitted to safety assessment prior to commercialisation. A concern related with PFS regards its botanical composition since unintentional swap of plants has been reported and also because adulterations by the substitution of higher cost botanicals for closely related, but cheaper species, can occur. Thus, there is a need for reliable methodologies to authenticate botanicals in commercialised PFS. Recently, molecular biology techniques have been suggested for this purpose. However, difficulties in recovering DNA from some PFS samples have been described (1). Thus, as part of a study for the botanical authentication of PFS, this work aimed at assessing the interference of pharmaceutical excipients on the recovery/amplification of DNA. Different PFS (tablets and capsules) were submitted to DNA extraction and amplified by real-time polymerase chain reaction (PCR) targeting universal eukaryotic and plant genes using species-specific primers for Hypericum DNA barcode loci. However, some samples gave consistently negative PCR amplifications irrespective of the target gene or DNA extraction method used, raising the question of whether some excipients could interfere with DNA extraction from PFS. To address this question, model mixtures of pharmaceutical excipients and water as control, were spiked with known amounts of template maize DNA. Each mixture was then submitted to DNA extraction and maize DNA quantified by real-time PCR. The use of either 10% talc or 0.5 % dyes (iron oxide or titanium dioxide) completely adsorbed DNA, resulting in negative PCR amplifications. The use of 1% talc or 10% silica, both frequently used as diluents in PFS, allowed recovering very low amounts of maize DNA (7.1 % and 2.5%, respectively). The results showed a clear adsorption phenomena that justify the hampering effect on DNA extraction from PFS explaining the inability of recovering DNA from some samples reported in previous works. Thus, a strategy to release plant DNA from excipients, allowing its extraction and further analysis was also assayed. Hypericum species were not detected in four PFS, although being described on the label.
Autores principais:Amaral, Joana S.
Outros Autores:Costa, Joana; Fernandes, Telmo J.R.; Batista, Andreia; Oliveira, Beatriz; Mafra, Isabel
Assunto:plant food supplements; botanical adulteration; molecular biology; excipients
Ano:2015
País:Portugal
Tipo de documento:documento de conferência
Tipo de acesso:acesso aberto
Instituição associada:Instituto Politécnico de Bragança
Idioma:inglês
Origem:Biblioteca Digital do IPB
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author Amaral, Joana S.
author2 Costa, Joana
Fernandes, Telmo J.R.
Batista, Andreia
Oliveira, Beatriz
Mafra, Isabel
author2_role author
author
author
author
author
author_facet Amaral, Joana S.
Costa, Joana
Fernandes, Telmo J.R.
Batista, Andreia
Oliveira, Beatriz
Mafra, Isabel
author_role author
contributor_name_str_mv Biblioteca Digital do IPB
country_str PT
creators_json_txt [{\"Person.name\":\"Amaral, Joana S.\",\"Person.identifier.orcid\":\"0000-0002-3648-7303\"},{\"Person.name\":\"Costa, Joana\"},{\"Person.name\":\"Fernandes, Telmo J.R.\"},{\"Person.name\":\"Batista, Andreia\"},{\"Person.name\":\"Oliveira, Beatriz\"},{\"Person.name\":\"Mafra, Isabel\"}]
datacite.contributors.contributor.contributorName.fl_str_mv Biblioteca Digital do IPB
datacite.creators.creator.creatorName.fl_str_mv Amaral, Joana S.
Costa, Joana
Fernandes, Telmo J.R.
Batista, Andreia
Oliveira, Beatriz
Mafra, Isabel
datacite.date.Accepted.fl_str_mv 2015-01-01T00:00:00Z
datacite.date.available.fl_str_mv 2018-04-04T11:32:54Z
datacite.date.embargoed.fl_str_mv 2018-04-04T11:32:54Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv plant food supplements; botanical adulteration; molecular biology; excipients
datacite.titles.title.fl_str_mv Detection of botanical adulterations in plant food supplements by molecular biology techniques
dc.contributor.none.fl_str_mv Biblioteca Digital do IPB
dc.creator.none.fl_str_mv Amaral, Joana S.
Costa, Joana
Fernandes, Telmo J.R.
Batista, Andreia
Oliveira, Beatriz
Mafra, Isabel
dc.date.Accepted.fl_str_mv 2015-01-01T00:00:00Z
dc.date.available.fl_str_mv 2018-04-04T11:32:54Z
dc.date.embargoed.fl_str_mv 2018-04-04T11:32:54Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv http://hdl.handle.net/10198/16672
dc.language.none.fl_str_mv eng
dc.rights.cclincense.fl_str_mv http://creativecommons.org/licenses/by/4.0/
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.subject.none.fl_str_mv plant food supplements; botanical adulteration; molecular biology; excipients
dc.title.fl_str_mv Detection of botanical adulterations in plant food supplements by molecular biology techniques
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_c94f
description In the last years, botanicals have become increasingly available in the EU market in the form of plant food supplements (PFS), which are legally considered as foods under Directive 2002/46/EC and consequently not submitted to safety assessment prior to commercialisation. A concern related with PFS regards its botanical composition since unintentional swap of plants has been reported and also because adulterations by the substitution of higher cost botanicals for closely related, but cheaper species, can occur. Thus, there is a need for reliable methodologies to authenticate botanicals in commercialised PFS. Recently, molecular biology techniques have been suggested for this purpose. However, difficulties in recovering DNA from some PFS samples have been described (1). Thus, as part of a study for the botanical authentication of PFS, this work aimed at assessing the interference of pharmaceutical excipients on the recovery/amplification of DNA. Different PFS (tablets and capsules) were submitted to DNA extraction and amplified by real-time polymerase chain reaction (PCR) targeting universal eukaryotic and plant genes using species-specific primers for Hypericum DNA barcode loci. However, some samples gave consistently negative PCR amplifications irrespective of the target gene or DNA extraction method used, raising the question of whether some excipients could interfere with DNA extraction from PFS. To address this question, model mixtures of pharmaceutical excipients and water as control, were spiked with known amounts of template maize DNA. Each mixture was then submitted to DNA extraction and maize DNA quantified by real-time PCR. The use of either 10% talc or 0.5 % dyes (iron oxide or titanium dioxide) completely adsorbed DNA, resulting in negative PCR amplifications. The use of 1% talc or 10% silica, both frequently used as diluents in PFS, allowed recovering very low amounts of maize DNA (7.1 % and 2.5%, respectively). The results showed a clear adsorption phenomena that justify the hampering effect on DNA extraction from PFS explaining the inability of recovering DNA from some samples reported in previous works. Thus, a strategy to release plant DNA from excipients, allowing its extraction and further analysis was also assayed. Hypericum species were not detected in four PFS, although being described on the label.
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funding.funder.alternateName_str_mv FCT
funding.funder.identifier_str_mv http://doi.org/10.13039/501100001871
funding.funder.name_str_mv Fundação para a Ciência e a Tecnologia
id ipb_c932af3f1e41b07d12c2cfaf660b630a
identifier.url.fl_str_mv http://hdl.handle.net/10198/16672
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instname_str Instituto Politécnico de Bragança
language eng
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oai_identifier_str oai:bibliotecadigital.ipb.pt:10198/16672
organization_str_mv urn:organizationAcronym:ipb
person_str_mv Amaral, Joana S.
Amaral, Joana S.
https://www.ciencia-id.pt/5319-7DE8-BEDA
5319-7DE8-BEDA
http://orcid.org/0000-0002-3648-7303
0000-0002-3648-7303
Costa, Joana
Fernandes, Telmo J.R.
Batista, Andreia
Oliveira, Beatriz
Mafra, Isabel
publishDate 2015
reponame_str Biblioteca Digital do IPB
repository_id_str urn:repositoryAcronym:ipb
service_str_mv urn:repositoryAcronym:ipb
spelling engpt_PTIn the last years, botanicals have become increasingly available in the EU market in the form of plant food supplements (PFS), which are legally considered as foods under Directive 2002/46/EC and consequently not submitted to safety assessment prior to commercialisation. A concern related with PFS regards its botanical composition since unintentional swap of plants has been reported and also because adulterations by the substitution of higher cost botanicals for closely related, but cheaper species, can occur. Thus, there is a need for reliable methodologies to authenticate botanicals in commercialised PFS. Recently, molecular biology techniques have been suggested for this purpose. However, difficulties in recovering DNA from some PFS samples have been described (1). Thus, as part of a study for the botanical authentication of PFS, this work aimed at assessing the interference of pharmaceutical excipients on the recovery/amplification of DNA. Different PFS (tablets and capsules) were submitted to DNA extraction and amplified by real-time polymerase chain reaction (PCR) targeting universal eukaryotic and plant genes using species-specific primers for Hypericum DNA barcode loci. However, some samples gave consistently negative PCR amplifications irrespective of the target gene or DNA extraction method used, raising the question of whether some excipients could interfere with DNA extraction from PFS. To address this question, model mixtures of pharmaceutical excipients and water as control, were spiked with known amounts of template maize DNA. Each mixture was then submitted to DNA extraction and maize DNA quantified by real-time PCR. The use of either 10% talc or 0.5 % dyes (iron oxide or titanium dioxide) completely adsorbed DNA, resulting in negative PCR amplifications. The use of 1% talc or 10% silica, both frequently used as diluents in PFS, allowed recovering very low amounts of maize DNA (7.1 % and 2.5%, respectively). The results showed a clear adsorption phenomena that justify the hampering effect on DNA extraction from PFS explaining the inability of recovering DNA from some samples reported in previous works. Thus, a strategy to release plant DNA from excipients, allowing its extraction and further analysis was also assayed. Hypericum species were not detected in four PFS, although being described on the label.application/pdfpt_PTDetection of botanical adulterations in plant food supplements by molecular biology techniquesPersonalAmaral, Joana S.DSpacehttp://dspace.org/items/42be2cf4-adc4-4e7f-ac60-7aab515b38cdDSpacehttp://dspace.org/items/42be2cf4-adc4-4e7f-ac60-7aab515b38cdAmaralJoana S.Ciência IDhttps://www.ciencia-id.pt5319-7DE8-BEDAORCIDhttp://orcid.org0000-0002-3648-7303Costa, JoanaFernandes, Telmo J.R.Batista, AndreiaOliveira, BeatrizMafra, IsabelHostingInstitutionOrganizationalBiblioteca Digital do IPBe-mailmailto:dspace@ipb.ptdspace@ipb.pt2018-04-04T11:32:54Z20152015-01-01T00:00:00ZHandlehttp://hdl.handle.net/10198/16672http://purl.org/coar/access_right/c_abf2open accessplant food supplements; botanical adulteration; molecular biology; excipients1563967 bytesFundação para a Ciência e a TecnologiaStructural features and immunoreactivity of plant food allergens: impact of technological food processing and in vitro digestibilityCrossref Funder IDhttp://doi.org/10.13039/501100001871other research producthttp://purl.org/coar/resource_type/c_c94fconference object2015http://creativecommons.org/licenses/by/4.0/http://purl.org/coar/access_right/c_abf2application/pdffulltexthttps://bibliotecadigital.ipb.pt/bitstreams/3cc9ccbb-02b8-4f50-a9a3-4b7af7d39f48/downloadEuroFoodChem XVIIIMadrid, Spain
spellingShingle Detection of botanical adulterations in plant food supplements by molecular biology techniques
Amaral, Joana S.
plant food supplements; botanical adulteration; molecular biology; excipients
status SINGLETON
subject.fl_str_mv plant food supplements; botanical adulteration; molecular biology; excipients
title Detection of botanical adulterations in plant food supplements by molecular biology techniques
title_full Detection of botanical adulterations in plant food supplements by molecular biology techniques
title_fullStr Detection of botanical adulterations in plant food supplements by molecular biology techniques
title_full_unstemmed Detection of botanical adulterations in plant food supplements by molecular biology techniques
title_short Detection of botanical adulterations in plant food supplements by molecular biology techniques
title_sort Detection of botanical adulterations in plant food supplements by molecular biology techniques
topic plant food supplements; botanical adulteration; molecular biology; excipients
topic_facet plant food supplements; botanical adulteration; molecular biology; excipients
url http://hdl.handle.net/10198/16672
visible 1