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Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study

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Resumo:The study’s aim was to synthesize a crystalline film formed by L-threonine crystals complexed with Cu2+ ions (LTCu) dispersed in a galactomannan (Gal) solution as well as to characterize its structural, vibrational, and thermal properties. Gal(LTCu) films were prepared by the addition of copper II L-threoninate crystals in concentrations of 0.25, 0.50, and 0.75 in 2%Gal solution. To characterize the Gal(LTCu) properties, we used X-ray diffraction (XRD), UV–Vis and Raman spectroscopy, thermogravimetry, and thermal analyses (TG- DTA). XRD showed that the Gal(LTCu) films are crystalline and have acquired coloration similar to the one of LTCu crystal. The UV–Vis spectra revealed that the films tend to assume a square planar conformation due to Jahn Teller effect. Bands related to the interaction between the metal ion with the organic compounds were observed through the Raman spectra. TG-DTA showed that the films exhibit low thermal stability due to the dehydration process
Autores principais:Oliveira Neto, João G.
Outros Autores:Cavalcante, Lincoln A.; Gomes, Eduardo S.; Dos Santos, Adenilson O.; Sousa, Francisco F; Mendes, Fernando 1973-; Macêdo, Ana Angélica M
Assunto:Crystalline films Threonine Copper Galactomannan solution
Ano:2019
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Instituto Politécnico de Coimbra
Idioma:inglês
Origem:Instituto Politécnico de Coimbra
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author Oliveira Neto, João G.
author2 Cavalcante, Lincoln A.
Gomes, Eduardo S.
Dos Santos, Adenilson O.
Sousa, Francisco F
Mendes, Fernando 1973-
Macêdo, Ana Angélica M
author2_role author
author
author
author
author
author
author_facet Oliveira Neto, João G.
Cavalcante, Lincoln A.
Gomes, Eduardo S.
Dos Santos, Adenilson O.
Sousa, Francisco F
Mendes, Fernando 1973-
Macêdo, Ana Angélica M
author_role author
contributor_name_str_mv Repositório Comum
country_str PT
creators_json_txt [{\"Person.name\":\"Oliveira Neto, João G.\"},{\"Person.name\":\"Cavalcante, Lincoln A.\"},{\"Person.name\":\"Gomes, Eduardo S.\"},{\"Person.name\":\"Dos Santos, Adenilson O.\"},{\"Person.name\":\"Sousa, Francisco F\"},{\"Person.name\":\"Mendes, Fernando 1973-\"},{\"Person.name\":\"Macêdo, Ana Angélica M\"}]
datacite.contributors.contributor.contributorName.fl_str_mv Repositório Comum
datacite.creators.creator.creatorName.fl_str_mv Oliveira Neto, João G.
Cavalcante, Lincoln A.
Gomes, Eduardo S.
Dos Santos, Adenilson O.
Sousa, Francisco F
Mendes, Fernando 1973-
Macêdo, Ana Angélica M
datacite.date.Accepted.fl_str_mv 2019-10-01T00:00:00Z
datacite.date.available.fl_str_mv 2020-04-17T21:39:36Z
datacite.date.embargoed.fl_str_mv 2020-04-17T21:39:36Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv Crystalline films
Threonine
Copper
Galactomannan solution
datacite.titles.title.fl_str_mv Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
dc.contributor.none.fl_str_mv Repositório Comum
dc.creator.none.fl_str_mv Oliveira Neto, João G.
Cavalcante, Lincoln A.
Gomes, Eduardo S.
Dos Santos, Adenilson O.
Sousa, Francisco F
Mendes, Fernando 1973-
Macêdo, Ana Angélica M
dc.date.Accepted.fl_str_mv 2019-10-01T00:00:00Z
dc.date.available.fl_str_mv 2020-04-17T21:39:36Z
dc.date.embargoed.fl_str_mv 2020-04-17T21:39:36Z
dc.format.none.fl_str_mv application/vnd.openxmlformats-officedocument.wordprocessingml.document
dc.identifier.none.fl_str_mv http://hdl.handle.net/10400.26/32016
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv Wiley
dc.rights.cclincense.fl_str_mv http://creativecommons.org/licenses/by-nc-sa/4.0/
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.subject.none.fl_str_mv Crystalline films
Threonine
Copper
Galactomannan solution
dc.title.fl_str_mv Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_6501
description The study’s aim was to synthesize a crystalline film formed by L-threonine crystals complexed with Cu2+ ions (LTCu) dispersed in a galactomannan (Gal) solution as well as to characterize its structural, vibrational, and thermal properties. Gal(LTCu) films were prepared by the addition of copper II L-threoninate crystals in concentrations of 0.25, 0.50, and 0.75 in 2%Gal solution. To characterize the Gal(LTCu) properties, we used X-ray diffraction (XRD), UV–Vis and Raman spectroscopy, thermogravimetry, and thermal analyses (TG- DTA). XRD showed that the Gal(LTCu) films are crystalline and have acquired coloration similar to the one of LTCu crystal. The UV–Vis spectra revealed that the films tend to assume a square planar conformation due to Jahn Teller effect. Bands related to the interaction between the metal ion with the organic compounds were observed through the Raman spectra. TG-DTA showed that the films exhibit low thermal stability due to the dehydration process
dirty 0
eu_rights_str_mv openAccess
format article
fulltext.url.fl_str_mv https://comum.rcaap.pt/bitstreams/bddb3d0d-be01-43a7-a70f-815440ad6801/download
id ipc_f4ace04e2ca910adbd55561ade52cfb8
identifier.url.fl_str_mv http://hdl.handle.net/10400.26/32016
instacron_str ipc
institution Instituto Politécnico de Coimbra
instname_str Instituto Politécnico de Coimbra
language eng
network_acronym_str ipc
network_name_str Instituto Politécnico de Coimbra
oai_identifier_str oai:comum.rcaap.pt:10400.26/32016
organization_str_mv urn:organizationAcronym:ipc
person_str_mv Oliveira Neto, João G.
Cavalcante, Lincoln A.
Gomes, Eduardo S.
Dos Santos, Adenilson O.
Sousa, Francisco F
Mendes, Fernando 1973-
Macêdo, Ana Angélica M
publishDate 2019
publisher.none.fl_str_mv Wiley
reponame_str Instituto Politécnico de Coimbra
repository_id_str urn:repositoryAcronym:ipc
service_str_mv urn:repositoryAcronym:ipc
spelling engWileypt_PTThe study’s aim was to synthesize a crystalline film formed by L-threonine crystals complexed with Cu2+ ions (LTCu) dispersed in a galactomannan (Gal) solution as well as to characterize its structural, vibrational, and thermal properties. Gal(LTCu) films were prepared by the addition of copper II L-threoninate crystals in concentrations of 0.25, 0.50, and 0.75 in 2%Gal solution. To characterize the Gal(LTCu) properties, we used X-ray diffraction (XRD), UV–Vis and Raman spectroscopy, thermogravimetry, and thermal analyses (TG- DTA). XRD showed that the Gal(LTCu) films are crystalline and have acquired coloration similar to the one of LTCu crystal. The UV–Vis spectra revealed that the films tend to assume a square planar conformation due to Jahn Teller effect. Bands related to the interaction between the metal ion with the organic compounds were observed through the Raman spectra. TG-DTA showed that the films exhibit low thermal stability due to the dehydration processapplication/vnd.openxmlformats-officedocument.wordprocessingml.documentpt_PTCrystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal studyOliveira Neto, João G.Cavalcante, Lincoln A.Gomes, Eduardo S.Dos Santos, Adenilson O.Sousa, Francisco FMendes, Fernando 1973-Macêdo, Ana Angélica MHostingInstitutionOrganizationalRepositório Comume-mailmailto:comum@rcaap.ptcomum@rcaap.ptISSNIsPartOf1548-2634DOIIsPartOf10.1002/pen.252602020-04-17T21:39:36Z2019-10-012019-10-01T00:00:00ZHandlehttp://hdl.handle.net/10400.26/32016http://purl.org/coar/access_right/c_abf2open accessCrystalline filmsThreonineCopperGalactomannan solution15475 bytesliteraturehttp://purl.org/coar/resource_type/c_6501journal article2019-10-01http://creativecommons.org/licenses/by-nc-sa/4.0/http://purl.org/coar/access_right/c_abf2application/vnd.openxmlformats-officedocument.wordprocessingml.documentfulltexthttps://comum.rcaap.pt/bitstreams/bddb3d0d-be01-43a7-a70f-815440ad6801/downloadPolymer Engineering & Science6017177
spellingShingle Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
Oliveira Neto, João G.
Crystalline films
Threonine
Copper
Galactomannan solution
status SINGLETON
subject.fl_str_mv Crystalline films
Threonine
Copper
Galactomannan solution
title Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
title_full Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
title_fullStr Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
title_full_unstemmed Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
title_short Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
title_sort Crystalline films of L‐threonine complexed with copper (II) dispersed in a Galactomannan solution: a structural, vibrational, and thermal study
topic Crystalline films
Threonine
Copper
Galactomannan solution
topic_facet Crystalline films
Threonine
Copper
Galactomannan solution
url http://hdl.handle.net/10400.26/32016
visible 1