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Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils

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Resumo:When considering complex scenarios involving several attributes, such as in environmental characterization, a clearer picture of reality can be achieved through the dimensional reduction of data. In this context, maps facilitate the visualization of spatial patterns of contaminant distribution and the identification of enriched areas. A set, of 15 Potentially Toxic Elements (PTEs) – (As, Ba, Cd, Co, Cr, Cu, Hg,Mo, Ni, Pb, Sb, Se, Tl, V, and Zn), was measured in soil, collected in Langreo's municipality (80 km2), Spain. Relative enrichment (RE) is introduced here to refer to the proportion of elements present in a given context. Indeed, a novel approach is provided for research into PTE fate. This method involves studying the variability of PTE proportions throughout the study area, thereby allowing the identification of dissemination trends. Traditional geostatistical approaches commonly use raw data (concentrations) accepting that the elements analyzedmake up the entirety of the soil. However, in geochemical studies the analyzed elements are just a fraction of the total soil composition. Therefore, considering compositional data is pivotal. The spatial characterization of PTEs considering raw and compositional data together allowed a broad discussion about, not only the PTEs concentration's distribution but also to reckon possible trends of relative enrichment (RE). Transformations to open closed data are widely used for this purpose. Spatial patterns have an indubitable interest. In this study, the Centered Log-ratio transformation (clr) was used, followed by its back-transformation, to build a set of compositional data that, combined with raw data, allowed to establish the sources of the PTEs and trends of spatial dissemination.
Autores principais:Boente, Carlos
Outros Autores:Albuquerque, M.T.D.; Fernández-Braña, A.; Gerassis, Saki; Sierra, C.; Gallego, J.R.
Assunto:Soil pollution PTEs Compositional data Ordinary kriging Local G-clustering Relative enrichment
Ano:2018
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Instituto Politécnico de Castelo Branco
Idioma:inglês
Origem:Repositório Científico do Instituto Politécnico de Castelo Branco
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author Boente, Carlos
author2 Albuquerque, M.T.D.
Fernández-Braña, A.
Gerassis, Saki
Sierra, C.
Gallego, J.R.
author2_role author
author
author
author
author
author_facet Boente, Carlos
Albuquerque, M.T.D.
Fernández-Braña, A.
Gerassis, Saki
Sierra, C.
Gallego, J.R.
author_role author
contributor_name_str_mv Repositório Científico do Instituto Politécnico de Castelo Branco
country_str PT
creators_json_txt [{\"Person.name\":\"Boente, Carlos\"},{\"Person.name\":\"Albuquerque, M.T.D.\",\"Person.identifier.orcid\":\"0000-0002-8782-6133\"},{\"Person.name\":\"Fernández-Braña, A.\"},{\"Person.name\":\"Gerassis, Saki\"},{\"Person.name\":\"Sierra, C.\"},{\"Person.name\":\"Gallego, J.R.\"}]
datacite.contributors.contributor.contributorName.fl_str_mv Repositório Científico do Instituto Politécnico de Castelo Branco
datacite.creators.creator.creatorName.fl_str_mv Boente, Carlos
Albuquerque, M.T.D.
Fernández-Braña, A.
Gerassis, Saki
Sierra, C.
Gallego, J.R.
datacite.date.Accepted.fl_str_mv 2018-01-01T00:00:00Z
datacite.date.available.fl_str_mv 2020-08-31T00:30:10Z
datacite.date.embargoed.fl_str_mv 2020-08-31T00:30:10Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv Soil pollution
PTEs
Compositional data
Ordinary kriging
Local G-clustering
Relative enrichment
datacite.titles.title.fl_str_mv Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
dc.contributor.none.fl_str_mv Repositório Científico do Instituto Politécnico de Castelo Branco
dc.creator.none.fl_str_mv Boente, Carlos
Albuquerque, M.T.D.
Fernández-Braña, A.
Gerassis, Saki
Sierra, C.
Gallego, J.R.
dc.date.Accepted.fl_str_mv 2018-01-01T00:00:00Z
dc.date.available.fl_str_mv 2020-08-31T00:30:10Z
dc.date.embargoed.fl_str_mv 2020-08-31T00:30:10Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv http://hdl.handle.net/10400.11/6046
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv Elsevier
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.subject.none.fl_str_mv Soil pollution
PTEs
Compositional data
Ordinary kriging
Local G-clustering
Relative enrichment
dc.title.fl_str_mv Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_6501
description When considering complex scenarios involving several attributes, such as in environmental characterization, a clearer picture of reality can be achieved through the dimensional reduction of data. In this context, maps facilitate the visualization of spatial patterns of contaminant distribution and the identification of enriched areas. A set, of 15 Potentially Toxic Elements (PTEs) – (As, Ba, Cd, Co, Cr, Cu, Hg,Mo, Ni, Pb, Sb, Se, Tl, V, and Zn), was measured in soil, collected in Langreo's municipality (80 km2), Spain. Relative enrichment (RE) is introduced here to refer to the proportion of elements present in a given context. Indeed, a novel approach is provided for research into PTE fate. This method involves studying the variability of PTE proportions throughout the study area, thereby allowing the identification of dissemination trends. Traditional geostatistical approaches commonly use raw data (concentrations) accepting that the elements analyzedmake up the entirety of the soil. However, in geochemical studies the analyzed elements are just a fraction of the total soil composition. Therefore, considering compositional data is pivotal. The spatial characterization of PTEs considering raw and compositional data together allowed a broad discussion about, not only the PTEs concentration's distribution but also to reckon possible trends of relative enrichment (RE). Transformations to open closed data are widely used for this purpose. Spatial patterns have an indubitable interest. In this study, the Centered Log-ratio transformation (clr) was used, followed by its back-transformation, to build a set of compositional data that, combined with raw data, allowed to establish the sources of the PTEs and trends of spatial dissemination.
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eu_rights_str_mv openAccess
format article
fulltext.url.fl_str_mv https://repositorio.ipcb.pt/bitstreams/51685812-fcfc-4cef-a4ff-87df82e37b92/download
id ripcb_bf64af09b94d3ecba09eac64868f967f
identifier.url.fl_str_mv http://hdl.handle.net/10400.11/6046
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oai_identifier_str oai:repositorio.ipcb.pt:10400.11/6046
organization_str_mv urn:organizationAcronym:ipcb
person_str_mv Boente, Carlos
Albuquerque, M.T.D.
Albuquerque, M.T.D.
https://www.ciencia-id.pt/5A1C-8956-4C0A
5A1C-8956-4C0A
http://orcid.org/0000-0002-8782-6133
0000-0002-8782-6133
Fernández-Braña, A.
Gerassis, Saki
Sierra, C.
Gallego, J.R.
publishDate 2018
publisher.none.fl_str_mv Elsevier
reponame_str Repositório Científico do Instituto Politécnico de Castelo Branco
repository_id_str urn:repositoryAcronym:ripcb
service_str_mv urn:repositoryAcronym:ripcb
spelling engElsevierpt_PTWhen considering complex scenarios involving several attributes, such as in environmental characterization, a clearer picture of reality can be achieved through the dimensional reduction of data. In this context, maps facilitate the visualization of spatial patterns of contaminant distribution and the identification of enriched areas. A set, of 15 Potentially Toxic Elements (PTEs) – (As, Ba, Cd, Co, Cr, Cu, Hg,Mo, Ni, Pb, Sb, Se, Tl, V, and Zn), was measured in soil, collected in Langreo's municipality (80 km2), Spain. Relative enrichment (RE) is introduced here to refer to the proportion of elements present in a given context. Indeed, a novel approach is provided for research into PTE fate. This method involves studying the variability of PTE proportions throughout the study area, thereby allowing the identification of dissemination trends. Traditional geostatistical approaches commonly use raw data (concentrations) accepting that the elements analyzedmake up the entirety of the soil. However, in geochemical studies the analyzed elements are just a fraction of the total soil composition. Therefore, considering compositional data is pivotal. The spatial characterization of PTEs considering raw and compositional data together allowed a broad discussion about, not only the PTEs concentration's distribution but also to reckon possible trends of relative enrichment (RE). Transformations to open closed data are widely used for this purpose. Spatial patterns have an indubitable interest. In this study, the Centered Log-ratio transformation (clr) was used, followed by its back-transformation, to build a set of compositional data that, combined with raw data, allowed to establish the sources of the PTEs and trends of spatial dissemination.application/pdfpt_PTCombining raw and compositional data to determine the spatial patterns of potentially toxic elements in soilsBoente, CarlosPersonalAlbuquerque, M.T.D.DSpacehttp://dspace.org/items/e2c2d171-e148-4c23-9cf8-0eb6d810c15eDSpacehttp://dspace.org/items/e2c2d171-e148-4c23-9cf8-0eb6d810c15eAlbuquerqueMaria TeresaCiência IDhttps://www.ciencia-id.pt5A1C-8956-4C0AORCIDhttp://orcid.org0000-0002-8782-6133Researcher IDhttps://www.researcherid.comB-1536-2013Scopus Author IDhttps://www.scopus.com55507421600Fernández-Braña, A.Gerassis, SakiSierra, C.Gallego, J.R.HostingInstitutionOrganizationalRepositório Científico do Instituto Politécnico de Castelo Brancoe-mailmailto:repositorio@ipcb.ptrepositorio@ipcb.ptISSNIsPartOf0048-9697DOIIsPartOf10.1016/j.scitotenv.2018.03.0482020-08-31T00:30:10Z20182018-01-01T00:00:00ZHandlehttp://hdl.handle.net/10400.11/6046http://purl.org/coar/access_right/c_abf2open accessSoil pollutionPTEsCompositional dataOrdinary krigingLocal G-clusteringRelative enrichment1384733 bytesliteraturehttp://purl.org/coar/resource_type/c_6501journal articlehttp://purl.org/coar/access_right/c_abf2application/pdffulltexthttps://repositorio.ipcb.pt/bitstreams/51685812-fcfc-4cef-a4ff-87df82e37b92/downloadScience of the Total Environment631-63211171126
spellingShingle Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
Boente, Carlos
Soil pollution
PTEs
Compositional data
Ordinary kriging
Local G-clustering
Relative enrichment
status SINGLETON
subject.fl_str_mv Soil pollution
PTEs
Compositional data
Ordinary kriging
Local G-clustering
Relative enrichment
title Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
title_full Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
title_fullStr Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
title_full_unstemmed Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
title_short Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
title_sort Combining raw and compositional data to determine the spatial patterns of potentially toxic elements in soils
topic Soil pollution
PTEs
Compositional data
Ordinary kriging
Local G-clustering
Relative enrichment
topic_facet Soil pollution
PTEs
Compositional data
Ordinary kriging
Local G-clustering
Relative enrichment
url http://hdl.handle.net/10400.11/6046
visible 1