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AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)

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Resumo:This work presents the AMD-precipitates from supergenic neoformation in a mine waste-dumps located in the North of Portugal (Penedono mine). The waste dumps resulted from exploitation of gold occurring in quartz veins with sulfides, mainly pyrite and arsenopyrite. As a result, the mine wastes are composed by detrital minerals, mainly quartz, feldspar, micas, and pyrite that coexist with supergenic phases, formed by evolution of the acid mine drainage solutions. Mineral-water interaction lead to neoformation processes, including salinization (formation of soluble salts efflorescences) and crustification, consisting of the layering of crusts of minerals deposited successively. Jarosite, scorodite, and several soluble salts, such as gypsum and rhomboclase were identified as the most abundant precipitates. In addition, mineralogical analyses revealed the abundant occurrence of poorly crystalline iron-oxyhydroxides as well as amorphous nanoprecipitates, mainly composed by iron and arsenic. Mobilization or fixation of toxic elements can be strongly regulated by these neoformation processes. The obtained results indicated that arsenic is retained either by crystalline phases, such as scorodite, or by amorphous iron arsenates. Jarosite also play an important role in controlling mobilization of metals and arsenic by assuring crustification of mine wastes.
Autores principais:Valente, Teresa Maria Fernandes
Outros Autores:Gomes, Patrícia; Santisteban, M.; Torre, M. L. de la; Grande, J. A.
Assunto:AMD-precipitates scorodite jarosite Penedono Portugal Precipitados-AMD scorodita
Ano:2016
País:Portugal
Tipo de documento:comunicação em conferência
Tipo de acesso:acesso restrito
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
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author Valente, Teresa Maria Fernandes
author2 Gomes, Patrícia
Santisteban, M.
Torre, M. L. de la
Grande, J. A.
author2_role author
author
author
author
author_facet Valente, Teresa Maria Fernandes
Gomes, Patrícia
Santisteban, M.
Torre, M. L. de la
Grande, J. A.
author_role author
contributor_name_str_mv RepositóriUM - Universidade do Minho
country_str PT
creators_json_txt [{\"Person.name\":\"Valente, Teresa Maria Fernandes\"},{\"Person.name\":\"Gomes, Patrícia\"},{\"Person.name\":\"Santisteban, M.\"},{\"Person.name\":\"Torre, M. L. de la\"},{\"Person.name\":\"Grande, J. A.\"}]
datacite.contributors.contributor.contributorName.fl_str_mv RepositóriUM - Universidade do Minho
datacite.creators.creator.creatorName.fl_str_mv Valente, Teresa Maria Fernandes
Gomes, Patrícia
Santisteban, M.
Torre, M. L. de la
Grande, J. A.
datacite.date.Accepted.fl_str_mv 2016-09-01T00:00:00Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_16ec
datacite.subjects.subject.fl_str_mv AMD-precipitates
scorodite
jarosite
Penedono
Portugal
Precipitados-AMD
scorodita
datacite.titles.title.fl_str_mv AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
Precipitados de drenaje ácido de mina en un ambiente rico en arsénico: el caso de la escombrera de Penedono (N Portugal)
dc.contributor.none.fl_str_mv RepositóriUM - Universidade do Minho
dc.creator.none.fl_str_mv Valente, Teresa Maria Fernandes
Gomes, Patrícia
Santisteban, M.
Torre, M. L. de la
Grande, J. A.
dc.date.Accepted.fl_str_mv 2016-09-01T00:00:00Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv https://hdl.handle.net/1822/50449
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv Sociedad Geológica de España
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_16ec
dc.subject.none.fl_str_mv AMD-precipitates
scorodite
jarosite
Penedono
Portugal
Precipitados-AMD
scorodita
dc.title.fl_str_mv AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
Precipitados de drenaje ácido de mina en un ambiente rico en arsénico: el caso de la escombrera de Penedono (N Portugal)
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_5794
description This work presents the AMD-precipitates from supergenic neoformation in a mine waste-dumps located in the North of Portugal (Penedono mine). The waste dumps resulted from exploitation of gold occurring in quartz veins with sulfides, mainly pyrite and arsenopyrite. As a result, the mine wastes are composed by detrital minerals, mainly quartz, feldspar, micas, and pyrite that coexist with supergenic phases, formed by evolution of the acid mine drainage solutions. Mineral-water interaction lead to neoformation processes, including salinization (formation of soluble salts efflorescences) and crustification, consisting of the layering of crusts of minerals deposited successively. Jarosite, scorodite, and several soluble salts, such as gypsum and rhomboclase were identified as the most abundant precipitates. In addition, mineralogical analyses revealed the abundant occurrence of poorly crystalline iron-oxyhydroxides as well as amorphous nanoprecipitates, mainly composed by iron and arsenic. Mobilization or fixation of toxic elements can be strongly regulated by these neoformation processes. The obtained results indicated that arsenic is retained either by crystalline phases, such as scorodite, or by amorphous iron arsenates. Jarosite also play an important role in controlling mobilization of metals and arsenic by assuring crustification of mine wastes.
dirty 0
eu_rights_str_mv restrictedAccess
format conferencePaper
fulltext.url.fl_str_mv https://repositorium.uminho.pt/bitstreams/f584d18f-895f-4196-bda0-0c609065a2c6/download
id rum_37985f7de062ac2c5dbe3b6de1d4bbbf
identifier.url.fl_str_mv https://hdl.handle.net/1822/50449
instacron_str repositorium
institution Universidade do Minho
instname_str Universidade do Minho
language eng
network_acronym_str rum
network_name_str RepositóriUM - Universidade do Minho
oai_identifier_str oai:repositorium.uminho.pt:1822/50449
organization_str_mv urn:organizationAcronym:repositorium
person_str_mv Valente, Teresa Maria Fernandes
Gomes, Patrícia
Santisteban, M.
Torre, M. L. de la
Grande, J. A.
publishDate 2016
publisher.none.fl_str_mv Sociedad Geológica de España
reponame_str RepositóriUM - Universidade do Minho
repository_id_str urn:repositoryAcronym:rum
service_str_mv urn:repositoryAcronym:rum
spelling engSociedad Geológica de EspañaporThis work presents the AMD-precipitates from supergenic neoformation in a mine waste-dumps located in the North of Portugal (Penedono mine). The waste dumps resulted from exploitation of gold occurring in quartz veins with sulfides, mainly pyrite and arsenopyrite. As a result, the mine wastes are composed by detrital minerals, mainly quartz, feldspar, micas, and pyrite that coexist with supergenic phases, formed by evolution of the acid mine drainage solutions. Mineral-water interaction lead to neoformation processes, including salinization (formation of soluble salts efflorescences) and crustification, consisting of the layering of crusts of minerals deposited successively. Jarosite, scorodite, and several soluble salts, such as gypsum and rhomboclase were identified as the most abundant precipitates. In addition, mineralogical analyses revealed the abundant occurrence of poorly crystalline iron-oxyhydroxides as well as amorphous nanoprecipitates, mainly composed by iron and arsenic. Mobilization or fixation of toxic elements can be strongly regulated by these neoformation processes. The obtained results indicated that arsenic is retained either by crystalline phases, such as scorodite, or by amorphous iron arsenates. Jarosite also play an important role in controlling mobilization of metals and arsenic by assuring crustification of mine wastes.application/pdfporAMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)AlternativeTitleporPrecipitados de drenaje ácido de mina en un ambiente rico en arsénico: el caso de la escombrera de Penedono (N Portugal)Valente, Teresa Maria FernandesGomes, PatríciaSantisteban, M.Torre, M. L. de laGrande, J. A.HostingInstitutionOrganizationalRepositóriUM - Universidade do Minhoe-mailmailto:repositorium@usdb.uminho.ptrepositorium@usdb.uminho.pt2016-092016-09-01T00:00:00ZHandlehttps://hdl.handle.net/1822/50449http://purl.org/coar/access_right/c_16ecrestricted accessAMD-precipitatesscoroditejarositePenedonoPortugalPrecipitados-AMDscorodita460294 bytesother research producthttp://purl.org/coar/resource_type/c_5794conference paperhttp://purl.org/coar/access_right/c_16ecapplication/pdffulltexthttps://repositorium.uminho.pt/bitstreams/f584d18f-895f-4196-bda0-0c609065a2c6/download
spellingShingle AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
Valente, Teresa Maria Fernandes
AMD-precipitates
scorodite
jarosite
Penedono
Portugal
Precipitados-AMD
scorodita
status SINGLETON
subject.fl_str_mv AMD-precipitates
scorodite
jarosite
Penedono
Portugal
Precipitados-AMD
scorodita
title AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
title_full AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
title_fullStr AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
title_full_unstemmed AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
title_short AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
title_sort AMD-precipitates formed in an arsenic-rich environment: the case of the Penedono mine waste-dumps (N Portugal)
topic AMD-precipitates
scorodite
jarosite
Penedono
Portugal
Precipitados-AMD
scorodita
topic_facet AMD-precipitates
scorodite
jarosite
Penedono
Portugal
Precipitados-AMD
scorodita
url https://hdl.handle.net/1822/50449
visible 1