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Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications

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Resumo:Polymer-based piezoelectric biomaterials have already proven their relevance for tissue engineering applications. Furthermore, the morphology of the scaffolds plays also an important role in cell proliferation and differentiation. The present work reports on poly(hydroxybutyrate-co-hydroxyvalerate) (PHBV), a biocompatible, biodegradable, and piezoelectric biopolymer that has been processed in different morphologies, including films, fibers, microspheres, and 3D scaffolds. The corresponding magnetically active PHBV-based composites were also produced. The effect of the morphology on physico-chemical, thermal, magnetic, and mechanical properties of pristine and composite samples was evaluated, as well as their cytotoxicity. It was observed that the morphology does not strongly affect the properties of the pristine samples but the introduction of cobalt ferrites induces changes in the degree of crystallinity that could affect the applicability of prepared biomaterials. Young’s modulus is dependent of the morphology and also increases with the addition of cobalt ferrites. Both pristine and PHBV/cobalt ferrite composite samples are not cytotoxic, indicating their suitability for tissue engineering applications.
Autores principais:Amaro, Luís
Outros Autores:Correia, D. M.; Marques-Almeida, Teresa; Martins, Pedro M.; Pérez, Leyre; Vilas, José L.; Botelho, Gabriela; Lanceros-Méndez, S.; Ribeiro, Clarisse
Assunto:Biomaterials Cobalt ferrites Poly(hydroxybutyrate-co-hydroxyvalerate) Tissue engineering
Ano:2018
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
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author Amaro, Luís
author2 Correia, D. M.
Marques-Almeida, Teresa
Martins, Pedro M.
Pérez, Leyre
Vilas, José L.
Botelho, Gabriela
Lanceros-Méndez, S.
Ribeiro, Clarisse
author2_role author
author
author
author
author
author
author
author
author_facet Amaro, Luís
Correia, D. M.
Marques-Almeida, Teresa
Martins, Pedro M.
Pérez, Leyre
Vilas, José L.
Botelho, Gabriela
Lanceros-Méndez, S.
Ribeiro, Clarisse
author_role author
contributor_name_str_mv Universidade do Minho
country_str PT
creators_json_str [{\"Person.name\":\"Amaro, Luís\"},{\"Person.name\":\"Correia, D. M.\"},{\"Person.name\":\"Marques-Almeida, Teresa\"},{\"Person.name\":\"Martins, Pedro M.\"},{\"Person.name\":\"Pérez, Leyre\"},{\"Person.name\":\"Vilas, José L.\"},{\"Person.name\":\"Botelho, Gabriela\"},{\"Person.name\":\"Lanceros-Méndez, S.\"},{\"Person.name\":\"Ribeiro, Clarisse\"}]
datacite.contributors.contributor.contributorName.fl_str_mv Universidade do Minho
datacite.creators.creator.creatorName.fl_str_mv Amaro, Luís
Correia, D. M.
Marques-Almeida, Teresa
Martins, Pedro M.
Pérez, Leyre
Vilas, José L.
Botelho, Gabriela
Lanceros-Méndez, S.
Ribeiro, Clarisse
datacite.date.Accepted.fl_str_mv 2018-07-24T00:00:00Z
datacite.date.available.fl_str_mv 2018-09-04T18:10:00Z
datacite.date.embargoed.fl_str_mv 2018-09-04T18:10:00Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv Biomaterials
Cobalt ferrites
Poly(hydroxybutyrate-co-hydroxyvalerate)
Tissue engineering
datacite.titles.title.fl_str_mv Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
dc.contributor.none.fl_str_mv Universidade do Minho
dc.creator.none.fl_str_mv Amaro, Luís
Correia, D. M.
Marques-Almeida, Teresa
Martins, Pedro M.
Pérez, Leyre
Vilas, José L.
Botelho, Gabriela
Lanceros-Méndez, S.
Ribeiro, Clarisse
dc.date.Accepted.fl_str_mv 2018-07-24T00:00:00Z
dc.date.available.fl_str_mv 2018-09-04T18:10:00Z
dc.date.embargoed.fl_str_mv 2018-09-04T18:10:00Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv https://hdl.handle.net/1822/55733
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv MDPI
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.subject.none.fl_str_mv Biomaterials
Cobalt ferrites
Poly(hydroxybutyrate-co-hydroxyvalerate)
Tissue engineering
dc.title.fl_str_mv Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_6501
description Polymer-based piezoelectric biomaterials have already proven their relevance for tissue engineering applications. Furthermore, the morphology of the scaffolds plays also an important role in cell proliferation and differentiation. The present work reports on poly(hydroxybutyrate-co-hydroxyvalerate) (PHBV), a biocompatible, biodegradable, and piezoelectric biopolymer that has been processed in different morphologies, including films, fibers, microspheres, and 3D scaffolds. The corresponding magnetically active PHBV-based composites were also produced. The effect of the morphology on physico-chemical, thermal, magnetic, and mechanical properties of pristine and composite samples was evaluated, as well as their cytotoxicity. It was observed that the morphology does not strongly affect the properties of the pristine samples but the introduction of cobalt ferrites induces changes in the degree of crystallinity that could affect the applicability of prepared biomaterials. Young’s modulus is dependent of the morphology and also increases with the addition of cobalt ferrites. Both pristine and PHBV/cobalt ferrite composite samples are not cytotoxic, indicating their suitability for tissue engineering applications.
dirty 0
eu_rights_str_mv openAccess
format article
fulltext.url.fl_str_mv https://prod-dspace.uminho.pt/bitstreams/728f23e9-2e8c-47fa-a1d1-e2e97a2cbcb0/download
id rum_53738e63c105a537896d07d47b3cbe21
identifier.url.fl_str_mv https://hdl.handle.net/1822/55733
instacron_str repositorium
institution Universidade do Minho
instname_str Universidade do Minho
language eng
network_acronym_str rum
network_name_str RepositóriUM - Universidade do Minho
oai_identifier_str oai:repositorium.uminho.pt:1822/55733
organization_str_mv urn:organizationAcronym:repositorium
person_str_mv Amaro, Luís
Correia, D. M.
Marques-Almeida, Teresa
Martins, Pedro M.
Pérez, Leyre
Vilas, José L.
Botelho, Gabriela
Lanceros-Méndez, S.
Ribeiro, Clarisse
publishDate 2018
publisher.none.fl_str_mv MDPI
reponame_str RepositóriUM - Universidade do Minho
repository_id_str urn:repositoryAcronym:rum
service_str_mv urn:repositoryAcronym:rum
spelling engMDPIporPolymer-based piezoelectric biomaterials have already proven their relevance for tissue engineering applications. Furthermore, the morphology of the scaffolds plays also an important role in cell proliferation and differentiation. The present work reports on poly(hydroxybutyrate-co-hydroxyvalerate) (PHBV), a biocompatible, biodegradable, and piezoelectric biopolymer that has been processed in different morphologies, including films, fibers, microspheres, and 3D scaffolds. The corresponding magnetically active PHBV-based composites were also produced. The effect of the morphology on physico-chemical, thermal, magnetic, and mechanical properties of pristine and composite samples was evaluated, as well as their cytotoxicity. It was observed that the morphology does not strongly affect the properties of the pristine samples but the introduction of cobalt ferrites induces changes in the degree of crystallinity that could affect the applicability of prepared biomaterials. Young’s modulus is dependent of the morphology and also increases with the addition of cobalt ferrites. Both pristine and PHBV/cobalt ferrite composite samples are not cytotoxic, indicating their suitability for tissue engineering applications.application/pdfengTailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applicationsAmaro, LuísCorreia, D. M.Marques-Almeida, TeresaMartins, Pedro M.Pérez, LeyreVilas, José L.Botelho, GabrielaLanceros-Méndez, S.Ribeiro, ClarisseHostingInstitutionOrganizationalUniversidade do Minhoe-mailmailto:repositorium@usdb.uminho.ptrepositorium@usdb.uminho.ptISSNIsPartOf1661-6596DOIIsPartOf10.3390/ijms190821492018-09-04T18:10:00Z2018-07-242018-09-04T16:56:10Z2018-07-24T00:00:00ZHandlehttps://hdl.handle.net/1822/55733http://purl.org/coar/access_right/c_abf2open accessBiomaterialsCobalt ferritesPoly(hydroxybutyrate-co-hydroxyvalerate)Tissue engineering5787897 bytesliteraturehttp://purl.org/coar/resource_type/c_6501journal articlehttp://purl.org/coar/access_right/c_abf2application/pdffulltexthttps://prod-dspace.uminho.pt/bitstreams/728f23e9-2e8c-47fa-a1d1-e2e97a2cbcb0/download
spellingShingle Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
Amaro, Luís
Biomaterials
Cobalt ferrites
Poly(hydroxybutyrate-co-hydroxyvalerate)
Tissue engineering
subject.fl_str_mv Biomaterials
Cobalt ferrites
Poly(hydroxybutyrate-co-hydroxyvalerate)
Tissue engineering
title Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
title_full Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
title_fullStr Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
title_full_unstemmed Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
title_short Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
title_sort Tailored biodegradable and electroactive poly(hydroxybutyrate-co-hydroxyvalerate) based morphologies for tissue engineering applications
topic Biomaterials
Cobalt ferrites
Poly(hydroxybutyrate-co-hydroxyvalerate)
Tissue engineering
topic_facet Biomaterials
Cobalt ferrites
Poly(hydroxybutyrate-co-hydroxyvalerate)
Tissue engineering
url https://hdl.handle.net/1822/55733
visible 1