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Grain size effect on self-mated CVD diamond dry tribosystems

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Resumo:Chemical vapour deposited (CVD) diamond coatings are important for tribological applications due to their unique combination of properties. Previous work demonstrated that silicon nitride (Si3N4) excels as a substrate for diamond coatings due to its low thermal expansion coefficient mismatch relative to diamond films resulting in a significant adhesion improvement. In this study, dense Si3N4 substrates were fabricated by pressureless sintering and diamond coated by microwave plasma chemical vapour deposition (MPCVD). The deposition time varied between 1 and 10 hours in order to investigate the effect of the diamond grain size and film thickness on the tribological behaviour of self-mated CVD diamond coatings on Si3N4. Reciprocating dry sliding ball-on-flat wear tests were performed in air up to 16 hours, at room temperature, with normal applied load ranging from 10 N to 105 N. The stroke and frequency of the sliding motion were kept constant with values of 6 mm and 1 Hz, respectively. Several characterisation techniques (SEM, AFM, micro-Raman) were used to identify the prevailing surface damage mechanisms. After a very short running-in regime, with high friction coefficients, a steady-state regime is reached, characterized by extremely low friction values (f~0.03). A mild wear mode was achieved for the longer runs, with wear coefficient values around 10-8 mm3N-1m-1. The larger grain sized and thicker coatings present smaller compressive residual stresses (below 1 GPa) due to a better in-depth accommodation of the contact pressure. This delays film delamination to much higher applied loads (105 N) than the thinner, small grain sized coatings, grown for 1 hour that fail in sliding under 35 N of normal load.
Autores principais:Abreu, C. S.
Outros Autores:Oliveira, F. J.; Belmonte, M.; Fernandes, A. J. S.; Silva, R. F.; Gomes, J. R.
Assunto:Wear Friction CVD diamond Grain size
Ano:2005
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
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author Abreu, C. S.
author2 Oliveira, F. J.
Belmonte, M.
Fernandes, A. J. S.
Silva, R. F.
Gomes, J. R.
author2_role author
author
author
author
author
author_facet Abreu, C. S.
Oliveira, F. J.
Belmonte, M.
Fernandes, A. J. S.
Silva, R. F.
Gomes, J. R.
author_role author
contributor_name_str_mv Universidade do Minho
country_str PT
creators_json_txt [{\"Person.name\":\"Abreu, C. S.\"},{\"Person.name\":\"Oliveira, F. J.\"},{\"Person.name\":\"Belmonte, M.\"},{\"Person.name\":\"Fernandes, A. J. S.\"},{\"Person.name\":\"Silva, R. F.\"},{\"Person.name\":\"Gomes, J. R.\"}]
datacite.contributors.contributor.contributorName.fl_str_mv Universidade do Minho
datacite.creators.creator.creatorName.fl_str_mv Abreu, C. S.
Oliveira, F. J.
Belmonte, M.
Fernandes, A. J. S.
Silva, R. F.
Gomes, J. R.
datacite.date.Accepted.fl_str_mv 2005-01-01T00:00:00Z
datacite.date.available.fl_str_mv 2007-02-08T11:28:40Z
datacite.date.embargoed.fl_str_mv 2007-02-08T11:28:40Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv Wear
Friction
CVD diamond
Grain size
datacite.titles.title.fl_str_mv Grain size effect on self-mated CVD diamond dry tribosystems
dc.contributor.none.fl_str_mv Universidade do Minho
dc.creator.none.fl_str_mv Abreu, C. S.
Oliveira, F. J.
Belmonte, M.
Fernandes, A. J. S.
Silva, R. F.
Gomes, J. R.
dc.date.Accepted.fl_str_mv 2005-01-01T00:00:00Z
dc.date.available.fl_str_mv 2007-02-08T11:28:40Z
dc.date.embargoed.fl_str_mv 2007-02-08T11:28:40Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv https://hdl.handle.net/1822/6128
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv Elsevier
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.subject.none.fl_str_mv Wear
Friction
CVD diamond
Grain size
dc.title.fl_str_mv Grain size effect on self-mated CVD diamond dry tribosystems
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_6501
description Chemical vapour deposited (CVD) diamond coatings are important for tribological applications due to their unique combination of properties. Previous work demonstrated that silicon nitride (Si3N4) excels as a substrate for diamond coatings due to its low thermal expansion coefficient mismatch relative to diamond films resulting in a significant adhesion improvement. In this study, dense Si3N4 substrates were fabricated by pressureless sintering and diamond coated by microwave plasma chemical vapour deposition (MPCVD). The deposition time varied between 1 and 10 hours in order to investigate the effect of the diamond grain size and film thickness on the tribological behaviour of self-mated CVD diamond coatings on Si3N4. Reciprocating dry sliding ball-on-flat wear tests were performed in air up to 16 hours, at room temperature, with normal applied load ranging from 10 N to 105 N. The stroke and frequency of the sliding motion were kept constant with values of 6 mm and 1 Hz, respectively. Several characterisation techniques (SEM, AFM, micro-Raman) were used to identify the prevailing surface damage mechanisms. After a very short running-in regime, with high friction coefficients, a steady-state regime is reached, characterized by extremely low friction values (f~0.03). A mild wear mode was achieved for the longer runs, with wear coefficient values around 10-8 mm3N-1m-1. The larger grain sized and thicker coatings present smaller compressive residual stresses (below 1 GPa) due to a better in-depth accommodation of the contact pressure. This delays film delamination to much higher applied loads (105 N) than the thinner, small grain sized coatings, grown for 1 hour that fail in sliding under 35 N of normal load.
dirty 0
eu_rights_str_mv openAccess
format article
fulltext.url.fl_str_mv https://prod-dspace.uminho.pt/bitstreams/fd477049-3949-4234-abb5-bfdb721ae4fb/download
id rum_6ec6545287ebcccda8a8fa24bc96fd1b
identifier.url.fl_str_mv https://hdl.handle.net/1822/6128
instacron_str repositorium
institution Universidade do Minho
instname_str Universidade do Minho
language eng
network_acronym_str rum
network_name_str RepositóriUM - Universidade do Minho
oai_identifier_str oai:repositorium.uminho.pt:1822/6128
organization_str_mv urn:organizationAcronym:repositorium
person_str_mv Abreu, C. S.
Oliveira, F. J.
Belmonte, M.
Fernandes, A. J. S.
Silva, R. F.
Gomes, J. R.
publishDate 2005
publisher.none.fl_str_mv Elsevier
reponame_str RepositóriUM - Universidade do Minho
repository_id_str urn:repositoryAcronym:rum
service_str_mv urn:repositoryAcronym:rum
spelling engElsevierengChemical vapour deposited (CVD) diamond coatings are important for tribological applications due to their unique combination of properties. Previous work demonstrated that silicon nitride (Si3N4) excels as a substrate for diamond coatings due to its low thermal expansion coefficient mismatch relative to diamond films resulting in a significant adhesion improvement. In this study, dense Si3N4 substrates were fabricated by pressureless sintering and diamond coated by microwave plasma chemical vapour deposition (MPCVD). The deposition time varied between 1 and 10 hours in order to investigate the effect of the diamond grain size and film thickness on the tribological behaviour of self-mated CVD diamond coatings on Si3N4. Reciprocating dry sliding ball-on-flat wear tests were performed in air up to 16 hours, at room temperature, with normal applied load ranging from 10 N to 105 N. The stroke and frequency of the sliding motion were kept constant with values of 6 mm and 1 Hz, respectively. Several characterisation techniques (SEM, AFM, micro-Raman) were used to identify the prevailing surface damage mechanisms. After a very short running-in regime, with high friction coefficients, a steady-state regime is reached, characterized by extremely low friction values (f~0.03). A mild wear mode was achieved for the longer runs, with wear coefficient values around 10-8 mm3N-1m-1. The larger grain sized and thicker coatings present smaller compressive residual stresses (below 1 GPa) due to a better in-depth accommodation of the contact pressure. This delays film delamination to much higher applied loads (105 N) than the thinner, small grain sized coatings, grown for 1 hour that fail in sliding under 35 N of normal load.application/pdfengGrain size effect on self-mated CVD diamond dry tribosystemsAbreu, C. S.Oliveira, F. J.Belmonte, M.Fernandes, A. J. S.Silva, R. F.Gomes, J. R.HostingInstitutionOrganizationalUniversidade do Minhoe-mailmailto:repositorium@usdb.uminho.ptrepositorium@usdb.uminho.ptISSNIsPartOf0043-1648DOIIsPartOf10.1016/j.wear.2005.01.0042007-02-08T11:28:40Z20052005-01-01T00:00:00ZHandlehttps://hdl.handle.net/1822/6128http://purl.org/coar/access_right/c_abf2open accessWearFrictionCVD diamondGrain size531390 bytesliteraturehttp://purl.org/coar/resource_type/c_6501journal articlehttp://purl.org/coar/access_right/c_abf2application/pdffulltexthttps://prod-dspace.uminho.pt/bitstreams/fd477049-3949-4234-abb5-bfdb721ae4fb/download
spellingShingle Grain size effect on self-mated CVD diamond dry tribosystems
Abreu, C. S.
Wear
Friction
CVD diamond
Grain size
status SINGLETON
subject.fl_str_mv Wear
Friction
CVD diamond
Grain size
title Grain size effect on self-mated CVD diamond dry tribosystems
title_full Grain size effect on self-mated CVD diamond dry tribosystems
title_fullStr Grain size effect on self-mated CVD diamond dry tribosystems
title_full_unstemmed Grain size effect on self-mated CVD diamond dry tribosystems
title_short Grain size effect on self-mated CVD diamond dry tribosystems
title_sort Grain size effect on self-mated CVD diamond dry tribosystems
topic Wear
Friction
CVD diamond
Grain size
topic_facet Wear
Friction
CVD diamond
Grain size
url https://hdl.handle.net/1822/6128
visible 1