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Electrically tunable interband collective excitations in biased bilayer and trilayer graphene

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Resumo:Collective excitations of charged particles under the influence of an electromagnetic field give rise to a rich variety of hybrid light-matter quasiparticles with unique properties. In metals, intraband collective response manifested by negative permittivity leads to plasmon polaritons with extreme field confinement, wavelength “squeezing,” and potentially low propagation losses. In contrast, photons in semiconductors commonly couple to interband collective response in the form of exciton polaritons, which give rise to completely different polaritonic properties, described by a superposition of the photon and exciton and an anti-crossing of the eigenstates. In this work, we identify the existence of plasmon-like collective excitations originating from the interband excitonic response of biased bilayer and trilayer graphene, in the form of graphene exciton polaritons (GEPs). We find that GEPs possess electrically tunable polaritonic properties and discover that such excitations follow a universal dispersion law for all surface polaritons in 2D excitonic systems. Accounting for nonlocal corrections to the excitonic response, we find that the GEPs exhibit confinement factors that can exceed those of graphene plasmons, and with moderate losses that would enable their observation in cryo-SNOM experiments. These predictions of plasmon-like interband collective excitations in biased graphene systems open up new research avenues for tunable plasmonic phenomena based on excitonic systems, and the ability to control and manipulate such phenomena at the atomic scale.
Autores principais:Eini, Tomer
Outros Autores:Quintela, M. F. C. Martins; Henriques, J. C. G.; Ribeiro, R. M.; Mazor, Yarden; Peres, N. M. R.; Epstein, Itai
Assunto:Excitons Plasmons Polaritons Quasi-particles & Collective excitations Surface plasmons Graphene
Ano:2025
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
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author Eini, Tomer
author2 Quintela, M. F. C. Martins
Henriques, J. C. G.
Ribeiro, R. M.
Mazor, Yarden
Peres, N. M. R.
Epstein, Itai
author2_role author
author
author
author
author
author
author_facet Eini, Tomer
Quintela, M. F. C. Martins
Henriques, J. C. G.
Ribeiro, R. M.
Mazor, Yarden
Peres, N. M. R.
Epstein, Itai
author_role author
contributor_name_str_mv Universidade do Minho
country_str PT
creators_json_txt [{\"Person.name\":\"Eini, Tomer\"},{\"Person.name\":\"Quintela, M. F. C. Martins\"},{\"Person.name\":\"Henriques, J. C. G.\"},{\"Person.name\":\"Ribeiro, R. M.\"},{\"Person.name\":\"Mazor, Yarden\"},{\"Person.name\":\"Peres, N. M. R.\"},{\"Person.name\":\"Epstein, Itai\"}]
datacite.contributors.contributor.contributorName.fl_str_mv Universidade do Minho
datacite.creators.creator.creatorName.fl_str_mv Eini, Tomer
Quintela, M. F. C. Martins
Henriques, J. C. G.
Ribeiro, R. M.
Mazor, Yarden
Peres, N. M. R.
Epstein, Itai
datacite.date.Accepted.fl_str_mv 2025-01-01T00:00:00Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv Excitons
Plasmons
Polaritons
Quasi-particles & Collective excitations
Surface plasmons
Graphene
datacite.titles.title.fl_str_mv Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
dc.contributor.none.fl_str_mv Universidade do Minho
dc.creator.none.fl_str_mv Eini, Tomer
Quintela, M. F. C. Martins
Henriques, J. C. G.
Ribeiro, R. M.
Mazor, Yarden
Peres, N. M. R.
Epstein, Itai
dc.date.Accepted.fl_str_mv 2025-01-01T00:00:00Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv https://hdl.handle.net/1822/100606
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv American Physical Society
dc.rights.cclincense.fl_str_mv http://creativecommons.org/licenses/by/4.0/
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.rights.rights.copyright.fl_str_mv openAccess
dc.subject.none.fl_str_mv Excitons
Plasmons
Polaritons
Quasi-particles & Collective excitations
Surface plasmons
Graphene
dc.title.fl_str_mv Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_6501
description Collective excitations of charged particles under the influence of an electromagnetic field give rise to a rich variety of hybrid light-matter quasiparticles with unique properties. In metals, intraband collective response manifested by negative permittivity leads to plasmon polaritons with extreme field confinement, wavelength “squeezing,” and potentially low propagation losses. In contrast, photons in semiconductors commonly couple to interband collective response in the form of exciton polaritons, which give rise to completely different polaritonic properties, described by a superposition of the photon and exciton and an anti-crossing of the eigenstates. In this work, we identify the existence of plasmon-like collective excitations originating from the interband excitonic response of biased bilayer and trilayer graphene, in the form of graphene exciton polaritons (GEPs). We find that GEPs possess electrically tunable polaritonic properties and discover that such excitations follow a universal dispersion law for all surface polaritons in 2D excitonic systems. Accounting for nonlocal corrections to the excitonic response, we find that the GEPs exhibit confinement factors that can exceed those of graphene plasmons, and with moderate losses that would enable their observation in cryo-SNOM experiments. These predictions of plasmon-like interband collective excitations in biased graphene systems open up new research avenues for tunable plasmonic phenomena based on excitonic systems, and the ability to control and manipulate such phenomena at the atomic scale.
dirty 0
eu_rights_str_mv openAccess
format article
fulltext.url.fl_str_mv https://repositorium.uminho.pt/bitstreams/91b708c9-d136-4143-9c48-eb1d44209ec2/download
funding.funder.alternateName_str_mv other
other
other
other
funding.funder.identifier_str_mv urn:openaire:ec__________::EC
urn:openaire:ec__________::EC
urn:openaire:fct_________::FCT
urn:openaire:fct_________::FCT
funding.funder.name_str_mv European Commission
European Commission
Fundação para a Ciência e a Tecnologia, I.P.
Fundação para a Ciência e a Tecnologia, I.P.
funding.identifier_str_mv 101078192
101129661
UIDB/04650/2020
PTDC/FIS-MAC/2045/2021
funding.name_str_mv HORIZON ERC Grants
HORIZON-ERC\HORIZON Action Grant Budget-Based
HORIZON EIC Grants
Concurso de avaliação no âmbito do Programa Plurianual de Financiamento de Unidades de I&D (2017/2018) - Financiamento Base
Concurso de Projetos IC&DT em Todos os Domínios Científicos
funding_str_mv 101078192
https://hdl.handle.net/1822/100616
101129661
https://hdl.handle.net/1822/100605
UIDB/04650/2020
https://hdl.handle.net/1822/97590
PTDC/FIS-MAC/2045/2021
https://hdl.handle.net/1822/98576
id rum_a7eb48351a331ebd2e51130fb8dfc51a
identifier.url.fl_str_mv https://hdl.handle.net/1822/100606
instacron_str repositorium
institution Universidade do Minho
instname_str Universidade do Minho
language eng
network_acronym_str rum
network_name_str RepositóriUM - Universidade do Minho
oai_identifier_str oai:repositorium.uminho.pt:1822/100606
organization_str_mv urn:organizationAcronym:repositorium
person_str_mv Eini, Tomer
Quintela, M. F. C. Martins
Henriques, J. C. G.
Ribeiro, R. M.
Mazor, Yarden
Peres, N. M. R.
Epstein, Itai
publishDate 2025
publisher.none.fl_str_mv American Physical Society
reponame_str RepositóriUM - Universidade do Minho
repository_id_str urn:repositoryAcronym:rum
service_str_mv urn:repositoryAcronym:rum
spelling engAmerican Physical SocietyengCollective excitations of charged particles under the influence of an electromagnetic field give rise to a rich variety of hybrid light-matter quasiparticles with unique properties. In metals, intraband collective response manifested by negative permittivity leads to plasmon polaritons with extreme field confinement, wavelength “squeezing,” and potentially low propagation losses. In contrast, photons in semiconductors commonly couple to interband collective response in the form of exciton polaritons, which give rise to completely different polaritonic properties, described by a superposition of the photon and exciton and an anti-crossing of the eigenstates. In this work, we identify the existence of plasmon-like collective excitations originating from the interband excitonic response of biased bilayer and trilayer graphene, in the form of graphene exciton polaritons (GEPs). We find that GEPs possess electrically tunable polaritonic properties and discover that such excitations follow a universal dispersion law for all surface polaritons in 2D excitonic systems. Accounting for nonlocal corrections to the excitonic response, we find that the GEPs exhibit confinement factors that can exceed those of graphene plasmons, and with moderate losses that would enable their observation in cryo-SNOM experiments. These predictions of plasmon-like interband collective excitations in biased graphene systems open up new research avenues for tunable plasmonic phenomena based on excitonic systems, and the ability to control and manipulate such phenomena at the atomic scale.application/pdfporElectrically tunable interband collective excitations in biased bilayer and trilayer grapheneEini, TomerQuintela, M. F. C. MartinsHenriques, J. C. G.Ribeiro, R. M.Mazor, YardenPeres, N. M. R.Epstein, ItaiHostingInstitutionOrganizationalUniversidade do Minhoe-mailmailto:repositorium@usdb.uminho.ptrepositorium@usdb.uminho.ptISSNIsPartOf0031-9007DOIIsPartOf10.1103/PhysRevLett.134.19690320252025-01-01T00:00:00ZHandlehttps://hdl.handle.net/1822/100606http://purl.org/coar/access_right/c_abf2open accessExcitonsPlasmonsPolaritonsQuasi-particles & Collective excitationsSurface plasmonsGraphene1626027 bytesEuropean CommissionTerahertz OPtoelectronics in BiLayer Graphene (101078192)HORIZON ERC GrantsHORIZON-ERC\HORIZON Action Grant Budget-Basedhttps://hdl.handle.net/1822/100616101078192Crossref Funder IDurn:openaire:ec__________::ECEuropean CommissionAdaptable bio-inspired polariton-polariton energy management (101129661)HORIZON EIC Grantshttps://hdl.handle.net/1822/100605101129661Crossref Funder IDurn:openaire:ec__________::ECFundação para a Ciência e a Tecnologia, I.P.Physics Center of Minho and Porto Universities (UIDB/04650/2020)Concurso de avaliação no âmbito do Programa Plurianual de Financiamento de Unidades de I&D (2017/2018) - Financiamento Basehttps://hdl.handle.net/1822/97590UIDB/04650/2020Crossref Funder IDurn:openaire:fct_________::FCTFundação para a Ciência e a Tecnologia, I.P.Excitations in quantum 2D materials (PTDC/FIS-MAC/2045/2021)Concurso de Projetos IC&DT em Todos os Domínios Científicoshttps://hdl.handle.net/1822/98576PTDC/FIS-MAC/2045/2021Crossref Funder IDurn:openaire:fct_________::FCTliteraturehttp://purl.org/coar/resource_type/c_6501journal article2025http://creativecommons.org/licenses/by/4.0/openAccesshttp://purl.org/coar/access_right/c_abf2application/pdffulltexthttps://repositorium.uminho.pt/bitstreams/91b708c9-d136-4143-9c48-eb1d44209ec2/download13418
spellingShingle Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
Eini, Tomer
Excitons
Plasmons
Polaritons
Quasi-particles & Collective excitations
Surface plasmons
Graphene
status SINGLETON
subject.fl_str_mv Excitons
Plasmons
Polaritons
Quasi-particles & Collective excitations
Surface plasmons
Graphene
title Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
title_full Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
title_fullStr Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
title_full_unstemmed Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
title_short Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
title_sort Electrically tunable interband collective excitations in biased bilayer and trilayer graphene
topic Excitons
Plasmons
Polaritons
Quasi-particles & Collective excitations
Surface plasmons
Graphene
topic_facet Excitons
Plasmons
Polaritons
Quasi-particles & Collective excitations
Surface plasmons
Graphene
url https://hdl.handle.net/1822/100606
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