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Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling

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Summary:Si1-xGex nanocrystals (NCs) of different composition and size were generated using the Molecular Dynamics (MD) method by minimizing NC’s total energy calculated using Tersoff’s empirical potential and applying rigid boundary conditions. The dynamical matrix of the relaxed NC was constructed and the NC phonon modes were calculated. The localisation of the principal (Si-Si, Si-Ge and Ge-Ge) modes is investigated by analysing their inverse participation ratio. The dependence of the corresponding Raman spectra, obtained by employing the bond polarisability model, upon x and the NC size is presented and compared to previous calculated results and available experimental data.
Main Authors:Vasin, Alexander
Other Authors:Vikhrova, Olga; Vasilevskiy, Mikhail
Subject:Nanocrystal Alloying Phonon Raman scattering
Year:2013
Country:Portugal
Document type:conference paper
Access type:open access
Associated institution:Universidade do Minho
Language:English
Origin:RepositóriUM - Universidade do Minho
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author Vasin, Alexander
author2 Vikhrova, Olga
Vasilevskiy, Mikhail
author2_role author
author
author_facet Vasin, Alexander
Vikhrova, Olga
Vasilevskiy, Mikhail
author_role author
contributor_name_str_mv RepositóriUM - Universidade do Minho
country_str PT
creators_json_txt [{\"Person.name\":\"Vasin, Alexander\"},{\"Person.name\":\"Vikhrova, Olga\"},{\"Person.name\":\"Vasilevskiy, Mikhail\"}]
datacite.contributors.contributor.contributorName.fl_str_mv RepositóriUM - Universidade do Minho
datacite.creators.creator.creatorName.fl_str_mv Vasin, Alexander
Vikhrova, Olga
Vasilevskiy, Mikhail
datacite.date.Accepted.fl_str_mv 2013-03-05T00:00:00Z
datacite.date.available.fl_str_mv 2014-01-03T09:53:39Z
datacite.date.embargoed.fl_str_mv 2014-01-03T09:53:39Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv Nanocrystal
Alloying
Phonon
Raman scattering
datacite.titles.title.fl_str_mv Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
dc.contributor.none.fl_str_mv RepositóriUM - Universidade do Minho
dc.creator.none.fl_str_mv Vasin, Alexander
Vikhrova, Olga
Vasilevskiy, Mikhail
dc.date.Accepted.fl_str_mv 2013-03-05T00:00:00Z
dc.date.available.fl_str_mv 2014-01-03T09:53:39Z
dc.date.embargoed.fl_str_mv 2014-01-03T09:53:39Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv https://hdl.handle.net/1822/27380
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv Wiley-VCH Verlag
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.subject.none.fl_str_mv Nanocrystal
Alloying
Phonon
Raman scattering
dc.title.fl_str_mv Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_5794
description Si1-xGex nanocrystals (NCs) of different composition and size were generated using the Molecular Dynamics (MD) method by minimizing NC’s total energy calculated using Tersoff’s empirical potential and applying rigid boundary conditions. The dynamical matrix of the relaxed NC was constructed and the NC phonon modes were calculated. The localisation of the principal (Si-Si, Si-Ge and Ge-Ge) modes is investigated by analysing their inverse participation ratio. The dependence of the corresponding Raman spectra, obtained by employing the bond polarisability model, upon x and the NC size is presented and compared to previous calculated results and available experimental data.
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eu_rights_str_mv openAccess
format conferencePaper
fulltext.url.fl_str_mv https://repositorium.uminho.pt/bitstreams/9e0f0390-a2b0-4657-ae6f-651258cc7c83/download
id rum_da4c81fbaac7b5ea6fa74751c3f4fe61
identifier.url.fl_str_mv https://hdl.handle.net/1822/27380
instacron_str repositorium
institution Universidade do Minho
instname_str Universidade do Minho
language eng
network_acronym_str rum
network_name_str RepositóriUM - Universidade do Minho
oai_identifier_str oai:repositorium.uminho.pt:1822/27380
organization_str_mv urn:organizationAcronym:repositorium
person_str_mv Vasin, Alexander
Vikhrova, Olga
Vasilevskiy, Mikhail
publishDate 2013
publisher.none.fl_str_mv Wiley-VCH Verlag
reponame_str RepositóriUM - Universidade do Minho
repository_id_str urn:repositoryAcronym:rum
service_str_mv urn:repositoryAcronym:rum
spelling engWiley-VCH VerlagporSi1-xGex nanocrystals (NCs) of different composition and size were generated using the Molecular Dynamics (MD) method by minimizing NC’s total energy calculated using Tersoff’s empirical potential and applying rigid boundary conditions. The dynamical matrix of the relaxed NC was constructed and the NC phonon modes were calculated. The localisation of the principal (Si-Si, Si-Ge and Ge-Ge) modes is investigated by analysing their inverse participation ratio. The dependence of the corresponding Raman spectra, obtained by employing the bond polarisability model, upon x and the NC size is presented and compared to previous calculated results and available experimental data.application/pdfporPhonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modellingVasin, AlexanderVikhrova, OlgaVasilevskiy, MikhailHostingInstitutionOrganizationalRepositóriUM - Universidade do Minhoe-mailmailto:repositorium@usdb.uminho.ptrepositorium@usdb.uminho.ptCITATIONPhys. Status Solidi C 10, No. 4, 701–704 (2013)ISSNIsPartOf1862-6270DOIIsPartOf10.1002/pssc.2012008012014-01-03T09:53:39Z2013-03-052012-10-072013-03-05T00:00:00ZHandlehttps://hdl.handle.net/1822/27380http://purl.org/coar/access_right/c_abf2open accessNanocrystalAlloyingPhononRaman scattering116426 bytesother research producthttp://purl.org/coar/resource_type/c_5794conference paperhttp://purl.org/coar/access_right/c_abf2application/pdffulltexthttps://repositorium.uminho.pt/bitstreams/9e0f0390-a2b0-4657-ae6f-651258cc7c83/download
spellingShingle Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
Vasin, Alexander
Nanocrystal
Alloying
Phonon
Raman scattering
status SINGLETON
subject.fl_str_mv Nanocrystal
Alloying
Phonon
Raman scattering
title Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
title_full Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
title_fullStr Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
title_full_unstemmed Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
title_short Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
title_sort Phonon modes and raman scattering in SixGe1-x nanocrystals: microscopic modelling
topic Nanocrystal
Alloying
Phonon
Raman scattering
topic_facet Nanocrystal
Alloying
Phonon
Raman scattering
url https://hdl.handle.net/1822/27380
visible 1