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Aligned silk-based 3-D architectures for contact guidance in tissue engineering

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Resumo:An important challenge in the biomaterials field is to mimic the structure of functional tissues via cell and extracellular matrix (ECM) alignment and anisotropy. Toward this goal, silk-based scaffolds resembling bone lamellar structure were developed using a freeze-drying technique. The structure could be controlled directly by solute concentration and freezing parameters, resulting in lamellar scaffolds with regular morphology. Different post-treatments, such as methanol, water annealing and steam sterilization, were investigated to induce water stability. The resulting structures exhibited significant differences in terms of morphological integrity, structure and mechanical properties. The lamellar thicknesses were ∼2.6 μm for the methanol-treated scaffolds and ∼5.8 μm for water-annealed. These values are in the range of those reported for human lamellar bone. Human bone marrow-derived mesenchymal stem cells (hMSC) were seeded on these silk fibroin lamellar scaffolds and grown under osteogenic conditions to assess the effect of the microstructure on cell behavior. Collagen in the newly deposited ECM was found aligned along the lamellar architectures. In the case of methanol-treated lamellar structures, the hMSC were able to migrate into the interior of the scaffolds, producing a multilamellar hybrid construct. The present morphology constitutes a useful pattern onto which hMSC cells attach and proliferate for guided formation of a highly oriented extracellular matrix.
Autores principais:Oliveira, A. L.
Outros Autores:Sun, L.; Kim, H. J.; Rice, W.; Kluge, J.; Reis, R. L.; Kaplan, David
Assunto:Freeze-drying Lamellar morphology cell alignment Silk scaffold Tissue engineering
Ano:2012
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
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author Oliveira, A. L.
author2 Sun, L.
Kim, H. J.
Rice, W.
Kluge, J.
Reis, R. L.
Kaplan, David
author2_role author
author
author
author
author
author
author_facet Oliveira, A. L.
Sun, L.
Kim, H. J.
Rice, W.
Kluge, J.
Reis, R. L.
Kaplan, David
author_role author
contributor_name_str_mv RepositóriUM - Universidade do Minho
country_str PT
creators_json_txt [{\"Person.name\":\"Oliveira, A. L.\"},{\"Person.name\":\"Sun, L.\"},{\"Person.name\":\"Kim, H. J.\"},{\"Person.name\":\"Rice, W.\"},{\"Person.name\":\"Kluge, J.\"},{\"Person.name\":\"Reis, R. L.\"},{\"Person.name\":\"Kaplan, David\"}]
datacite.contributors.contributor.contributorName.fl_str_mv RepositóriUM - Universidade do Minho
datacite.creators.creator.creatorName.fl_str_mv Oliveira, A. L.
Sun, L.
Kim, H. J.
Rice, W.
Kluge, J.
Reis, R. L.
Kaplan, David
datacite.date.Accepted.fl_str_mv 2012-03-01T00:00:00Z
datacite.date.available.fl_str_mv 2013-04-10T14:36:37Z
datacite.date.embargoed.fl_str_mv 2013-04-10T14:36:37Z
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv Freeze-drying
Lamellar morphology cell alignment
Silk scaffold
Tissue engineering
datacite.titles.title.fl_str_mv Aligned silk-based 3-D architectures for contact guidance in tissue engineering
dc.contributor.none.fl_str_mv RepositóriUM - Universidade do Minho
dc.creator.none.fl_str_mv Oliveira, A. L.
Sun, L.
Kim, H. J.
Rice, W.
Kluge, J.
Reis, R. L.
Kaplan, David
dc.date.Accepted.fl_str_mv 2012-03-01T00:00:00Z
dc.date.available.fl_str_mv 2013-04-10T14:36:37Z
dc.date.embargoed.fl_str_mv 2013-04-10T14:36:37Z
dc.format.none.fl_str_mv application/pdf
dc.identifier.none.fl_str_mv https://hdl.handle.net/1822/23652
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv Elsevier
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.subject.none.fl_str_mv Freeze-drying
Lamellar morphology cell alignment
Silk scaffold
Tissue engineering
dc.title.fl_str_mv Aligned silk-based 3-D architectures for contact guidance in tissue engineering
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_6501
description An important challenge in the biomaterials field is to mimic the structure of functional tissues via cell and extracellular matrix (ECM) alignment and anisotropy. Toward this goal, silk-based scaffolds resembling bone lamellar structure were developed using a freeze-drying technique. The structure could be controlled directly by solute concentration and freezing parameters, resulting in lamellar scaffolds with regular morphology. Different post-treatments, such as methanol, water annealing and steam sterilization, were investigated to induce water stability. The resulting structures exhibited significant differences in terms of morphological integrity, structure and mechanical properties. The lamellar thicknesses were ∼2.6 μm for the methanol-treated scaffolds and ∼5.8 μm for water-annealed. These values are in the range of those reported for human lamellar bone. Human bone marrow-derived mesenchymal stem cells (hMSC) were seeded on these silk fibroin lamellar scaffolds and grown under osteogenic conditions to assess the effect of the microstructure on cell behavior. Collagen in the newly deposited ECM was found aligned along the lamellar architectures. In the case of methanol-treated lamellar structures, the hMSC were able to migrate into the interior of the scaffolds, producing a multilamellar hybrid construct. The present morphology constitutes a useful pattern onto which hMSC cells attach and proliferate for guided formation of a highly oriented extracellular matrix.
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eu_rights_str_mv openAccess
format article
fulltext.url.fl_str_mv https://repositorium.uminho.pt/bitstreams/5da29b4d-711c-4cce-834c-58235e017231/download
id rum_e99fe1ee2a2fc67b2df3b2a36d0206cc
identifier.url.fl_str_mv https://hdl.handle.net/1822/23652
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institution Universidade do Minho
instname_str Universidade do Minho
language eng
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oai_identifier_str oai:repositorium.uminho.pt:1822/23652
organization_str_mv urn:organizationAcronym:repositorium
person_str_mv Oliveira, A. L.
Sun, L.
Kim, H. J.
Rice, W.
Kluge, J.
Reis, R. L.
Kaplan, David
publishDate 2012
publisher.none.fl_str_mv Elsevier
reponame_str RepositóriUM - Universidade do Minho
repository_id_str urn:repositoryAcronym:rum
service_str_mv urn:repositoryAcronym:rum
spelling engElsevierporAn important challenge in the biomaterials field is to mimic the structure of functional tissues via cell and extracellular matrix (ECM) alignment and anisotropy. Toward this goal, silk-based scaffolds resembling bone lamellar structure were developed using a freeze-drying technique. The structure could be controlled directly by solute concentration and freezing parameters, resulting in lamellar scaffolds with regular morphology. Different post-treatments, such as methanol, water annealing and steam sterilization, were investigated to induce water stability. The resulting structures exhibited significant differences in terms of morphological integrity, structure and mechanical properties. The lamellar thicknesses were ∼2.6 μm for the methanol-treated scaffolds and ∼5.8 μm for water-annealed. These values are in the range of those reported for human lamellar bone. Human bone marrow-derived mesenchymal stem cells (hMSC) were seeded on these silk fibroin lamellar scaffolds and grown under osteogenic conditions to assess the effect of the microstructure on cell behavior. Collagen in the newly deposited ECM was found aligned along the lamellar architectures. In the case of methanol-treated lamellar structures, the hMSC were able to migrate into the interior of the scaffolds, producing a multilamellar hybrid construct. The present morphology constitutes a useful pattern onto which hMSC cells attach and proliferate for guided formation of a highly oriented extracellular matrix.application/pdfporAligned silk-based 3-D architectures for contact guidance in tissue engineeringOliveira, A. L.Sun, L.Kim, H. J.Rice, W.Kluge, J.Reis, R. L.Kaplan, DavidHostingInstitutionOrganizationalRepositóriUM - Universidade do Minhoe-mailmailto:repositorium@usdb.uminho.ptrepositorium@usdb.uminho.ptPMID22202909ISSNIsPartOf1742-7061DOIIsPartOf10.1016/j.actbio.2011.12.0152013-04-10T14:36:37Z2012-032012-032013-04-10T10:37:07Z2012-03-01T00:00:00ZHandlehttps://hdl.handle.net/1822/23652http://purl.org/coar/access_right/c_abf2open accessFreeze-dryingLamellar morphology cell alignmentSilk scaffoldTissue engineering3382853 bytesliteraturehttp://purl.org/coar/resource_type/c_6501journal articlehttp://purl.org/coar/access_right/c_abf2application/pdffulltexthttps://repositorium.uminho.pt/bitstreams/5da29b4d-711c-4cce-834c-58235e017231/download
spellingShingle Aligned silk-based 3-D architectures for contact guidance in tissue engineering
Oliveira, A. L.
Freeze-drying
Lamellar morphology cell alignment
Silk scaffold
Tissue engineering
status SINGLETON
subject.fl_str_mv Freeze-drying
Lamellar morphology cell alignment
Silk scaffold
Tissue engineering
title Aligned silk-based 3-D architectures for contact guidance in tissue engineering
title_full Aligned silk-based 3-D architectures for contact guidance in tissue engineering
title_fullStr Aligned silk-based 3-D architectures for contact guidance in tissue engineering
title_full_unstemmed Aligned silk-based 3-D architectures for contact guidance in tissue engineering
title_short Aligned silk-based 3-D architectures for contact guidance in tissue engineering
title_sort Aligned silk-based 3-D architectures for contact guidance in tissue engineering
topic Freeze-drying
Lamellar morphology cell alignment
Silk scaffold
Tissue engineering
topic_facet Freeze-drying
Lamellar morphology cell alignment
Silk scaffold
Tissue engineering
url https://hdl.handle.net/1822/23652
visible 1