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Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment

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Resumo:Electrochemical monitoring techniques were employed in this study to assess anticorrosion performance of Phyllanthus muellerianus leaf-extract on concrete steel- reinforcement in 0.5 M H2SO4, used for simulating industrial/microbial environment. For this, steel-reinforced concretes admixed with different concentrations of the natural plant leaf-extract were partially immersed in the acidic test-solution and subjected to electrochemical monitoring of corrosion potential, corrosion current and corrosion rate. Test responses analysed as per ASTM G16-95 R04, showed that the corrosion rate correlated, r = 84.93%, ANOVA p-value = 0.0403, with the leaf-extract concentration admixed in concrete and the ratio of the standard deviation of potential to the standard deviation of current. These identified the 0.3333% Phyllanthus muellerianus (per weight of cement) with optimum effectiveness at inhibiting steel-reinforcement corrosion both by the experimental model, η = 91.66 & pm;2.51%, and by the prediction from the correlation fitting model, η = 85.54 & pm;14.44%. Fittings of both the experimental and the predicted data followed the Flory-Huggins and the Frumkin adsorption isotherms which suggest prevalent mechanism of physical adsorption (physisorption) of the extract on steel-rebar surface. These support the use of Phyllanthus muellerianus as environmentally-friendly admixture for inhibiting concrete steel-reinforcement corrosion in the industrial/microbial service-environment.
Autores principais:Okeniyi,Joshua O.
Outros Autores:Loto,Cleophas A.; Popoola,Abimbola P. I.
Assunto:steel-rebar corrosion in acidic environment environmentally-friendly inhibitor correlation fitting analysis inhibition efficiency adsorption isotherm
Ano:2014
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Fundação para a Ciência e Tecnologia
Idioma:inglês
Origem:SciELO Portugal
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author Okeniyi,Joshua O.
author2 Loto,Cleophas A.
Popoola,Abimbola P. I.
author2_role author
author
author_facet Okeniyi,Joshua O.
Loto,Cleophas A.
Popoola,Abimbola P. I.
author_role author
country_str PT
creators_json_txt [{\"Person.name\":\"Okeniyi,Joshua O.\"},{\"Person.name\":\"Loto,Cleophas A.\"},{\"Person.name\":\"Popoola,Abimbola P. I.\"}]
datacite.creators.creator.creatorName.fl_str_mv Okeniyi,Joshua O.
Loto,Cleophas A.
Popoola,Abimbola P. I.
datacite.rights.fl_str_mv http://purl.org/coar/access_right/c_abf2
datacite.subjects.subject.fl_str_mv steel-rebar corrosion in acidic environment
environmentally-friendly inhibitor
correlation fitting analysis
inhibition efficiency
adsorption isotherm
datacite.titles.title.fl_str_mv Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
dc.creator.none.fl_str_mv Okeniyi,Joshua O.
Loto,Cleophas A.
Popoola,Abimbola P. I.
dc.format.none.fl_str_mv text/html
dc.identifier.none.fl_str_mv http://scielo.pt/scielo.php?script=sci_arttext&pid=S0872-19042014000300002
dc.language.none.fl_str_mv eng
dc.publisher.none.fl_str_mv Sociedade Portuguesa de Electroquímica
dc.rights.none.fl_str_mv http://purl.org/coar/access_right/c_abf2
dc.source.none.fl_str_mv Portugaliae Electrochimica Acta v.32 n.3 2014
dc.subject.none.fl_str_mv steel-rebar corrosion in acidic environment
environmentally-friendly inhibitor
correlation fitting analysis
inhibition efficiency
adsorption isotherm
dc.title.fl_str_mv Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
dc.type.none.fl_str_mv http://purl.org/coar/resource_type/c_6501
description Electrochemical monitoring techniques were employed in this study to assess anticorrosion performance of Phyllanthus muellerianus leaf-extract on concrete steel- reinforcement in 0.5 M H2SO4, used for simulating industrial/microbial environment. For this, steel-reinforced concretes admixed with different concentrations of the natural plant leaf-extract were partially immersed in the acidic test-solution and subjected to electrochemical monitoring of corrosion potential, corrosion current and corrosion rate. Test responses analysed as per ASTM G16-95 R04, showed that the corrosion rate correlated, r = 84.93%, ANOVA p-value = 0.0403, with the leaf-extract concentration admixed in concrete and the ratio of the standard deviation of potential to the standard deviation of current. These identified the 0.3333% Phyllanthus muellerianus (per weight of cement) with optimum effectiveness at inhibiting steel-reinforcement corrosion both by the experimental model, η = 91.66 & pm;2.51%, and by the prediction from the correlation fitting model, η = 85.54 & pm;14.44%. Fittings of both the experimental and the predicted data followed the Flory-Huggins and the Frumkin adsorption isotherms which suggest prevalent mechanism of physical adsorption (physisorption) of the extract on steel-rebar surface. These support the use of Phyllanthus muellerianus as environmentally-friendly admixture for inhibiting concrete steel-reinforcement corrosion in the industrial/microbial service-environment.
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person_str_mv Okeniyi,Joshua O.
Loto,Cleophas A.
Popoola,Abimbola P. I.
publishDate 2014
publisher.none.fl_str_mv Sociedade Portuguesa de Electroquímica
reponame_str SciELO Portugal
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spelling Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environmentOkeniyi,Joshua O.Loto,Cleophas A.Popoola,Abimbola P. I.steel-rebar corrosion in acidic environmentenvironmentally-friendly inhibitorcorrelation fitting analysisinhibition efficiencyadsorption isothermopen accesshttp://purl.org/coar/access_right/c_abf2http://scielo.pt/scielo.php?script=sci_arttext&pid=S0872-19042014000300002URLhttp://scielo.pt/scielo.php?script=sci_arttext&pid=S0872-19042014000300002URLHasVersion2014-05-01Electrochemical monitoring techniques were employed in this study to assess anticorrosion performance of Phyllanthus muellerianus leaf-extract on concrete steel- reinforcement in 0.5 M H2SO4, used for simulating industrial/microbial environment. For this, steel-reinforced concretes admixed with different concentrations of the natural plant leaf-extract were partially immersed in the acidic test-solution and subjected to electrochemical monitoring of corrosion potential, corrosion current and corrosion rate. Test responses analysed as per ASTM G16-95 R04, showed that the corrosion rate correlated, r = 84.93%, ANOVA p-value = 0.0403, with the leaf-extract concentration admixed in concrete and the ratio of the standard deviation of potential to the standard deviation of current. These identified the 0.3333% Phyllanthus muellerianus (per weight of cement) with optimum effectiveness at inhibiting steel-reinforcement corrosion both by the experimental model, η = 91.66 & pm;2.51%, and by the prediction from the correlation fitting model, η = 85.54 & pm;14.44%. Fittings of both the experimental and the predicted data followed the Flory-Huggins and the Frumkin adsorption isotherms which suggest prevalent mechanism of physical adsorption (physisorption) of the extract on steel-rebar surface. These support the use of Phyllanthus muellerianus as environmentally-friendly admixture for inhibiting concrete steel-reinforcement corrosion in the industrial/microbial service-environment.Sociedade Portuguesa de ElectroquímicaPortugaliae Electrochimica Acta v.32 n.3 2014text/htmlengjournal articlehttp://purl.org/coar/resource_type/c_6501literature
spellingShingle Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
Okeniyi,Joshua O.
steel-rebar corrosion in acidic environment
environmentally-friendly inhibitor
correlation fitting analysis
inhibition efficiency
adsorption isotherm
status SINGLETON
subject.fl_str_mv steel-rebar corrosion in acidic environment
environmentally-friendly inhibitor
correlation fitting analysis
inhibition efficiency
adsorption isotherm
title Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
title_full Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
title_fullStr Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
title_full_unstemmed Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
title_short Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
title_sort Electrochemical Performance of Phyllanthus Muellerianus on the Corrosion of Concrete Steel-reinforcement in Industrial/Microbial Simulating-environment
topic steel-rebar corrosion in acidic environment
environmentally-friendly inhibitor
correlation fitting analysis
inhibition efficiency
adsorption isotherm
topic_facet steel-rebar corrosion in acidic environment
environmentally-friendly inhibitor
correlation fitting analysis
inhibition efficiency
adsorption isotherm
url http://scielo.pt/scielo.php?script=sci_arttext&pid=S0872-19042014000300002
visible 1