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Radical-type reactions in protic and aprotic media : comparisons in nickel-catalysed electrochemical reductive cyclisations

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Detalhes bibliográficos
Resumo:The electrochemical reductive cyclisation of unsaturated organic halides in the presence of Ni(II) complexes as catalysts was examined in aprotic solvents such as DMF and in protic solvents such as ethanol, butanol or ethanolewater mixtures. The presence of the alcohol media enhanced the rate of recycling of the catalytic species.
Autores principais:Dunach, E.
Outros Autores:Esteves, Ana Paula; Medeiros, Maria José; Neves, C. S. S.; Olivero, S.
Assunto:Electrosynthesis Ethanol Cyclisation Radical Nickel Tetrahydrofuran
Ano:2009
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:The electrochemical reductive cyclisation of unsaturated organic halides in the presence of Ni(II) complexes as catalysts was examined in aprotic solvents such as DMF and in protic solvents such as ethanol, butanol or ethanolewater mixtures. The presence of the alcohol media enhanced the rate of recycling of the catalytic species.