Publicação
Ag fractals formed on top of a porous TiO2 thin film
| Resumo: | This work demonstrates the formation of Ag fractals on top of a Ag:TiO2 thin film. The dendrite-type objects emerged from a homogeneous and highly transparent Ag:TiO2 nanocomposite, via the mechanism of diffusion-limited-aggregation of Ag atoms, during heat-treatment at 500 ºC. A porous TiO2 matrix was also formed during this process, opening a wide range of possible applications, namely in sensing-based ones, together with surface enhanced spectroscopies. Furthermore, fractals incorporate a wide range of shapes and spatial scales, inducing a potentially interesting optical response, over the whole visible range, presumably related with localized surface plasmon modes with very broad spectral distribution. |
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| Autores principais: | Borges, Joel Nuno Pinto |
| Outros Autores: | Rodrigues, M. S.; Lopes, C.; Costa, D.; Ferreira, A.; Pereira, Rui M. S.; Costa, M. F.; Vasilevskiy, Mikhail; Vaz, F. |
| Assunto: | Silver fractals TiO2 Surface Plasmon Resonance Diffusion-Limited Aggregation silver fractals |
| Ano: | 2016 |
| País: | Portugal |
| Tipo de documento: | artigo |
| Tipo de acesso: | acesso aberto |
| Instituição associada: | Universidade do Minho |
| Idioma: | inglês |
| Origem: | RepositóriUM - Universidade do Minho |
| Resumo: | This work demonstrates the formation of Ag fractals on top of a Ag:TiO2 thin film. The dendrite-type objects emerged from a homogeneous and highly transparent Ag:TiO2 nanocomposite, via the mechanism of diffusion-limited-aggregation of Ag atoms, during heat-treatment at 500 ºC. A porous TiO2 matrix was also formed during this process, opening a wide range of possible applications, namely in sensing-based ones, together with surface enhanced spectroscopies. Furthermore, fractals incorporate a wide range of shapes and spatial scales, inducing a potentially interesting optical response, over the whole visible range, presumably related with localized surface plasmon modes with very broad spectral distribution. |
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