Publicação

Synthesis and characterization of formyl-thienylpyridazines as versatile precursors for several optical applications

Ver documento

Detalhes bibliográficos
Resumo:Novel thienylpyridazines 3-4 functionalized with the formyl group on the aryl or heteroaryl moieties were synthesized through Suzuki coupling of bromo-thienylpyridazine 2 with commercially available (hetero)aryl-boronic acids. On the other hand precursor 2 was prepared by reaction of thienylpyridazinone 1 with POBr3. The new heterocyclic systems 3-4 were characterised by the usual spectroscopic techniques. In the future, these versatile formyl precursors will be further functionalized and characterized in order to evaluate their potential application as novel NLO-chromophores or as dyes sensitizers for DSSCs.
Autores principais:Fernandes, Sara S. M.
Outros Autores:Raposo, M. Manuela M.
Assunto:Heterocyclic aldehydes Pyridazine Suzuki coupling pi-conjugated systems Nonlinear optics (NLO) Dye-sensitized solar cells (DSSC) Synthesis Ciências Naturais::Ciências Químicas
Ano:2013
País:Portugal
Tipo de documento:outro
Tipo de acesso:acesso restrito
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:Novel thienylpyridazines 3-4 functionalized with the formyl group on the aryl or heteroaryl moieties were synthesized through Suzuki coupling of bromo-thienylpyridazine 2 with commercially available (hetero)aryl-boronic acids. On the other hand precursor 2 was prepared by reaction of thienylpyridazinone 1 with POBr3. The new heterocyclic systems 3-4 were characterised by the usual spectroscopic techniques. In the future, these versatile formyl precursors will be further functionalized and characterized in order to evaluate their potential application as novel NLO-chromophores or as dyes sensitizers for DSSCs.