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Push-pull tricyanovinyl-substituted thienylpyrroles: synthesis, solvatochromic and electrochemical properties

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Detalhes bibliográficos
Resumo:New tricyanovinyl- derivatives 1 of 1-(alkyl)aryl-2-(2'-thienyl)pyrroles 2 have been synthesized and characterized. Compounds 1 display dramatic reductions in both their optical and electrochemical band gaps in comparison to thienylpyrroles 2. The solvatochomic behavior of tricyanovinyl- derivatives 1 was investigated in a variety of solvents. In agreement with the solvatochromic and the electrochemical studies for push-pull derivatives I the new compounds prepared, can find application for manufacturing new materials with notable non-linear optical properties.
Autores principais:Raposo, M. Manuela M.
Outros Autores:Sousa, Ana M. R. C.; Fonseca, A. Maurício C.; Kirsch, G.
Assunto:Thiophene Pyrrole Push-pull thienylpyrroles Tricyanovinylation UV-visible spectroscopy Chromophores Solvatochromism Electrochemistry Non-linear optical (NLO) material
Ano:2006
País:Portugal
Tipo de documento:comunicação em conferência
Tipo de acesso:acesso restrito
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:New tricyanovinyl- derivatives 1 of 1-(alkyl)aryl-2-(2'-thienyl)pyrroles 2 have been synthesized and characterized. Compounds 1 display dramatic reductions in both their optical and electrochemical band gaps in comparison to thienylpyrroles 2. The solvatochomic behavior of tricyanovinyl- derivatives 1 was investigated in a variety of solvents. In agreement with the solvatochromic and the electrochemical studies for push-pull derivatives I the new compounds prepared, can find application for manufacturing new materials with notable non-linear optical properties.