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New thienylpyrrolyl-cyanoacetic acid derivatives: synthesis and evaluation of the optical and solvatochromic properties

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Detalhes bibliográficos
Resumo:The novel thienylpyrrolyl-cyanoacetic acid derivatives were obtained in good yields through a simple Knoevenagel condensation of the corresponding precursor aldehydes with cyanoacetic acid in acetonitrile at reflux, using piperidine as catalyst. The formyl precursors 1-2 were obtained through two different methods: (i) lithiation followed by treatment with DMF and (ii) Suzuki cross-coupling reaction. The novel push-pull systems were completely characterized by the usual spectroscopic techniques and the optical and solvatochromic properties were evaluated.
Autores principais:Batista, R. M. F
Outros Autores:Costa, Susana P. G.; Raposo, M. Manuela M.
Assunto:Thiophene Pyrrole Cyanoacetic acids UV-visible spectroscopy Solvatochromism Fluorescence Synthesis Heterocycles nonlinear optics (NLO) Dye sensitized solar cells (DSSCs)
Ano:2017
País:Portugal
Tipo de documento:comunicação em conferência
Tipo de acesso:acesso aberto
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:The novel thienylpyrrolyl-cyanoacetic acid derivatives were obtained in good yields through a simple Knoevenagel condensation of the corresponding precursor aldehydes with cyanoacetic acid in acetonitrile at reflux, using piperidine as catalyst. The formyl precursors 1-2 were obtained through two different methods: (i) lithiation followed by treatment with DMF and (ii) Suzuki cross-coupling reaction. The novel push-pull systems were completely characterized by the usual spectroscopic techniques and the optical and solvatochromic properties were evaluated.