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Role of ultraviolet absorbers (UVA) and hindered amine light stabilizers (HALS) in ABS stabilization

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Resumo:The present work evaluates the combination effect of hindered amine light stabilizers (HALS) and ultraviolet absorbers (UVA) on the ultraviolet (UV) stability of acrylonitrilebutadiene- styrene (ABS). Thus, two types of light stabilizers, Tinuvin P and Chimassorb 119 FL, were used to improve the ABS endurance against UV. Stabilized ABS samples were submitted to accelerated weathering in a Xenontest 150 S chamber, according to standard methods, in order to predict copolymer lifetime within a commercially acceptable time period. Infrared spectroscopy with attenuated total reflectance accessory (FTIR-ATR) was used to follow chemical modifications that occur on the material surface as a consequence of degradation process. While non-stabilized ABS samples loose the butadiene component in the first 22 h of exposure, in stabilized samples submitted to same accelerated conditions this component only disappears after 150 h of exposure. Non-stabilized and stabilized ABS samples present a similar yellowing behavior, a gradually increase with exposure time. Nevertheless, as expected, color modifications are less pronounced for stabilized ABS samples. The results obtained suggest that a better performance was achieved for stabilized ABS samples with Tinuvin P and Chimassorb 119 FL, which is very important to extend the copolymer lifetime.
Autores principais:Santos, R. M.
Outros Autores:Botelho, Gabriela; Machado, A. V.
Assunto:ABS Light stabilizers Yellowing Chemical modifications
Ano:2010
País:Portugal
Tipo de documento:comunicação em conferência
Tipo de acesso:acesso restrito
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:The present work evaluates the combination effect of hindered amine light stabilizers (HALS) and ultraviolet absorbers (UVA) on the ultraviolet (UV) stability of acrylonitrilebutadiene- styrene (ABS). Thus, two types of light stabilizers, Tinuvin P and Chimassorb 119 FL, were used to improve the ABS endurance against UV. Stabilized ABS samples were submitted to accelerated weathering in a Xenontest 150 S chamber, according to standard methods, in order to predict copolymer lifetime within a commercially acceptable time period. Infrared spectroscopy with attenuated total reflectance accessory (FTIR-ATR) was used to follow chemical modifications that occur on the material surface as a consequence of degradation process. While non-stabilized ABS samples loose the butadiene component in the first 22 h of exposure, in stabilized samples submitted to same accelerated conditions this component only disappears after 150 h of exposure. Non-stabilized and stabilized ABS samples present a similar yellowing behavior, a gradually increase with exposure time. Nevertheless, as expected, color modifications are less pronounced for stabilized ABS samples. The results obtained suggest that a better performance was achieved for stabilized ABS samples with Tinuvin P and Chimassorb 119 FL, which is very important to extend the copolymer lifetime.