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5´-alkoxy-2,2´-bithiophene azo dyes: a novel promising series of NLO chromophores

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Detalhes bibliográficos
Resumo:A series of bithienyl azo dyes has been prepared from their corresponding coupling components, 5-alkoxy-2,2´-bithiophenes. The solvatochromic behavior of the compounds was investigated. The hyperpolarizabilities β of derivatives 3-5 were measured using hyper-Rayleigh scattering and thermogravimetric analysis (TGA) was used to evaluate their thermal stability. The experimental results indicate that, good nonlinearity-thermal stability is well balanced for azo-bithiophene NLO-chromophores 3-5 making them good candidates for NLO applications.
Autores principais:Raposo, M. Manuela M.
Outros Autores:Ferreira, Ana M. P. F.; Belsley, M.; Moura, João C. V. P.
Assunto:Synthesis Azo coupling 5-alkoxy-2,2´-bithiophene couplers Heterocyclic azo dyes Solvatochromic probes UV-visible spectroscopy Thermal stability Nonlinear optics (NLO) applications Donor-acceptor conjugated systems First hyperpolarizability nonlinear optics (NLO)
Ano:2008
País:Portugal
Tipo de documento:artigo
Tipo de acesso:acesso aberto
Instituição associada:Universidade do Minho
Idioma:inglês
Origem:RepositóriUM - Universidade do Minho
Descrição
Resumo:A series of bithienyl azo dyes has been prepared from their corresponding coupling components, 5-alkoxy-2,2´-bithiophenes. The solvatochromic behavior of the compounds was investigated. The hyperpolarizabilities β of derivatives 3-5 were measured using hyper-Rayleigh scattering and thermogravimetric analysis (TGA) was used to evaluate their thermal stability. The experimental results indicate that, good nonlinearity-thermal stability is well balanced for azo-bithiophene NLO-chromophores 3-5 making them good candidates for NLO applications.